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Stimuli-Responsive Liquid Crystal Printheads for Spatial and Temporal Control of Polymerization.

Xin Wang, Hao Sun, Young-Ki Kim, Daniel B Wright, Michael Tsuei, Nathan C Gianneschi, Nicholas L Abbott,

Polymerization reactions triggered by stimuli play a pivotal role in material science, with applications ranging from lithography to biomedicine to adaptive materials. However, the development of chemically-triggered, stimuli-responsive systems that can confer spatial and temporal control on polymerization remains a challenge. Herein, chemical stimuli-induced polymerization based on a liquid crystal ... Read more >>

Adv Mater (Advanced materials (Deerfield Beach, Fla.))
[2022, :e2106535]

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Ultra-high electrical conductivity in filler-free polymeric hydrogels toward thermoelectrics and electromagnetic interference shielding.

Jing Wang, Qing Li, Kuncai Li, Xu Sun, Yizhuo Wang, Tiantian Zhuang, Junjie Yan, Hong Wang,

xxxx. This article is protected by copyright. All rights reserved. ... Read more >>

Adv Mater (Advanced materials (Deerfield Beach, Fla.))
[2022, :e2109904]

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Electrical Tuning of Plasmonic Conducting Polymer Nanoantennas.

Akchheta Karki, Giancarlo Cincotti, Shangzhi Chen, Vallery Stanishev, Vanya Darakchieva, Chuanfei Wang, Mats Fahlman, Magnus P Jonsson,

Nanostructures of conventional metals offer manipulation of light at the nanoscale but are largely limited to static behavior due to fixed material properties. To develop the next frontier of dynamic nanooptics and metasurfaces, we utilize the redox-tunable optical properties of conducting polymers, as recently shown capable of sustaining plasmons in ... Read more >>

Adv Mater (Advanced materials (Deerfield Beach, Fla.))
[2022, :e2107172]

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Ultrasensitive and Robust 120 keV Hard X-ray Imaging Detector Based on Mixed-Halide Perovskite CsPbBr3-n In Single Crystals.

Peng Zhang, Yunqiu Hua, Yadong Xu, Qihao Sun, Xiang Li, Fucai Cui, Lin Liu, Yanxiao Bi, Guodong Zhang, Xutang Tao,

The relatively low resistivity and severe ion migration in inorganic perovskite CsPbBr3 significantly degrade the performance of X-ray detectors due to their high detection limit and current drift. We investigate the electrical properties and X-ray detection performances of CsPbBr3-n In single crystals by doping the iodine atoms into the melt-grown ... Read more >>

Adv Mater (Advanced materials (Deerfield Beach, Fla.))
[2022, :e2106562]

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A Tissue Adhesion-Controllable and Biocompatible Small-scale Hydrogel Adhesive Robot.

Yun-Woo Lee, Sungwoo Chun, Donghoon Son, Xinghao Hu, Martina Schneider, Metin Sitti,

xxxx. This article is protected by copyright. All rights reserved. ... Read more >>

Adv Mater (Advanced materials (Deerfield Beach, Fla.))
[2022, :e2109325]

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Monolithic Perovskite-silicon Tandem Solar cells: from the Lab to Fab?

Fan Fu, Jia Li, Terry Chien-Jen Yang, Haoming Liang, Antonin Faes, Quentin Jeangros, Christophe Ballif, Yi Hou,

This review focuses on monolithic 2-terminal perovskite-silicon tandem solar cells and discusses key scientific and technological challenges to address in view of an industrial implementation of this technology. We start by examining the different crystalline silicon (c-Si) technologies suitable for pairing with perovskites, followed by reviewing recent developments in the ... Read more >>

Adv Mater (Advanced materials (Deerfield Beach, Fla.))
[2022, :e2106540]

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Biomimetic Human lung-on-a-chip with Colorful Displaying Microphysiological Breath.

Yujuan Zhu, Lingyu Sun, Yu Wang, Lijun Cai, Zhuohao Zhang, Yixuan Shang, Yuanjin Zhao,

Lung-on-a-chip models hold great promise for disease modeling and drug screening in the past decade. Herein, inspired by the iridescence phenomenon of soap bubbles, we present a novel biomimetic 3D microphysiological lung-on-a-chip system with breathing visuality. The system with an array of pulmonary alveoli at the physiological scale was constructed ... Read more >>

Adv Mater (Advanced materials (Deerfield Beach, Fla.))
[2022, :e2108972]

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Electrostatically Driven Polarization Flop and strain-induced Curvature in free-standing Ferroelectric Superlattices.

Yaqi Li, Edoardo Zatterin, Michele Conroy, Anastasiia Pylypets, Fedir Borodavka, Alexander Björling, Dirk J Groenendijk, Edouard Lesne, Adam J Clancy, Marios Hadjimichael, Demie Kepaptsoglou, Quentin Ramasse, Andrea Caviglia, Jiri Hlinka, Ursel Bangert, Steven Leake, Pavlo Zubko,

The combination of strain and electrostatic engineering in epitaxial heterostructures of ferroelectric oxides offers many possibilities for inducing new phases, complex polar topologies, and enhanced electrical properties. However, the dominant effect of substrate clamping can also limit the electromechanical response and often leaves electrostatics to play a secondary role. Releasing ... Read more >>

Adv Mater (Advanced materials (Deerfield Beach, Fla.))
[2022, :e2106826]

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Optical Rashba effect in a light-emitting perovskite metasurface.

Jingyi Tian, Giorgio Adamo, Hailong Liu, Maciej Klein, Song Han, Hong Liu, Cesare Soci,

XXXXXXXXXXXXX This article is protected by copyright. All rights reserved. ... Read more >>

Adv Mater (Advanced materials (Deerfield Beach, Fla.))
[2022, :e2109157]

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Co-Delivery of Precisely Prescribed Multi-Prodrug Combination by Engineered Nanocarrier Enables Efficient Individualized Cancer Chemotherapy.

Yuqiang Li, Yitong Jiang, Ziyan Zheng, Nan Du, Shuli Guan, Wenxuan Guo, Xiaohu Tang, Jiajunzi Cui, Lanqiong Zhang, Kunpeng Liu, Qingsong Yu, Zhihua Gan,

The limited anticancer drug library and the frequent occurrence of drug resistance have driven monotherapy-based cancer therapy into a difficult situation. Considering the formidable process of new drug discovery, combination therapy using currently available drugs is a potential alternative. Nevertheless, the barrier between in vitro combination screening and precise in ... Read more >>

Adv Mater (Advanced materials (Deerfield Beach, Fla.))
[2022, :e2110490]

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Immuno-Engineered Nanodecoys for the Multi-Target Anti-Inflammatory Treatment of Autoimmune Diseases.

Mengying Hou, Yuansong Wei, Ziyin Zhao, Wenqing Han, Renxiang Zhou, Yang Zhou, Yiran Zheng, Lichen Yin,

Over-activated T cells and over-produced pro-inflammatory cytokines form a self-amplified signaling loop to continuously exacerbate the dysregulated inflammatory response and propel the progression of autoimmune diseases (AIDs). Herein, immuno-engineered nanodecoys (NDs) based on poly(lactic-co-glycolic acid) nanoparticles (PLGA NPs) coated with PD-L1-expressing macrophage membrane (PRM) were developed to mediate multi-target interruption ... Read more >>

Adv Mater (Advanced materials (Deerfield Beach, Fla.))
[2022, :e2108817]

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Retina-Inspired Color-Cognitive Learning via Chromatically Controllable Mixed Quantum Dot Synaptic Transistor Arrays.

Chanho Jo, Jaehyun Kim, Jee Young Kwak, Sung Min Kwon, Joon Bee Park, Jeehoon Kim, Gyeong-Su Park, Myung-Gil Kim, Yong-Hoon Kim, Sung Kyu Park,

Artificial photonic synapses are emerging as a promising implementation to emulate the human visual cognitive system by consolidating a series of processes for sensing and memorizing visual information into one system. In particular, mimicking retinal functions such as multispectral color perception and controllable nonvolatility is important for realizing artificial visual ... Read more >>

Adv Mater (Advanced materials (Deerfield Beach, Fla.))
[2022, :e2108979]

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A Ferrotoroidic Candidate with Well-separated Spin Chains.

Jun Zhang, Xiancheng Wang, Long Zhou, Gangxiu Liu, Devashibhai T Adroja, Ivan da Silva, Franz Demmel, Dmitry Khalyavin, Jhuma Sannigrahi, Hari S Nair, Lei Duan, Jianfa Zhao, Zeng Deng, Runze Yu, Xi Shen, Richeng Yu, Hui Zhao, Jimin Zhao, Youwen Long, Zhiwei Hu, Hong-Ji Lin, Ting-Shan Chan, Chien-Te Chen, Wei Wu, Changqing Jin,

The search of novel quasi one-dimensional (1D) materials is one of the important aspects in the field of material science. Toroidal moment, the order parameter of ferrotoroidic order, can be generated by a head-to-tail configuration of magnetic moment. It has been theoretically proposed that one-dimensional (1D) dimerized and antiferromagnetic-like spin ... Read more >>

Adv Mater (Advanced materials (Deerfield Beach, Fla.))
[2022, :e2106728]

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Multilayer Reservoir Computing Based on Ferroelectric α-In2 Se3 for Hierarchical Information Processing.

Keqin Liu, Bingjie Dang, Teng Zhang, Zhen Yang, Lin Bao, Liying Xu, Caidie Cheng, Ru Huang, Yuchao Yang,

Dynamic physical systems such as reservoir computing (RC) architectures have shown great prospect in temporal information processing, whereas hierarchical information processing capability is still lacking due to the absence of advanced multilayer reservoir elements. Here, a stackable reservoir system is constructed based on ferroelectric α-In2 Se3 devices with voltage input ... Read more >>

Adv Mater (Advanced materials (Deerfield Beach, Fla.))
[2022, :e2108826]

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Two Dimensional Covalent Organic Frameworks: From Synthetic Strategies to Advanced optical-electrical-magnetic Functionalities.

Congyong Wang, Zhicheng Zhang, Yating Zhu, Chenhuai Yang, Jishan Wu, Wenping Hu,

Covalent organic frameworks (COFs), an emerging class of organic crystalline polymers with highly oriented structures and permanent porosity, can adopt two-dimensional (2D) or three-dimensional (3D) architectures depending on the different topological diagrams of the monomers. Notably, 2D COFs have particularly gained much attention due to the extraordinary merits of their ... Read more >>

Adv Mater (Advanced materials (Deerfield Beach, Fla.))
[2022, :e2102290]

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Andreev Interference in the Surface Accumulation Layer of Half-Shell InAsSb/Al Hybrid Nanowires.

Lukas Stampfer, Damon J Carrad, Dags Olsteins, Christian E N Petersen, Sabbir A Khan, Peter Krogstrup, Thomas S Jespersen,

Understanding the spatial distribution of charge carriers in III-V nanowires proximity coupled to superconductors is important for the design and interpretation of experiments based on hybrid quantum devices. In this letter, the gate-dependent surface accumulation layer of half-shell InAsSb/Al nanowires was studied by means of Andreev interference in a parallel magnetic ... Read more >>

Adv Mater (Advanced materials (Deerfield Beach, Fla.))
[2022, :e2108878]

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Bistability, Remanence, Read/write-memory and Logic Gate Function via A Stimuli Responsive Polymer.

Joanna Michalska-Walkowiak, Beate Förster, Stephan Hauschild, Stephan Förster,

Stimuli responsive materials change their state in response to external triggers. Switching between different states enables to write, store and read information, if the transition between the states exhibits hysteresis. Thermally responsive polymers exhibit an intrinsic hysteresis for the volume phase transition between the swollen and de-swollen solution state. We ... Read more >>

Adv Mater (Advanced materials (Deerfield Beach, Fla.))
[2022, :e2108833]

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Full-flexible Intelligent Thermal Touch Panel Based on Intrinsically Plastic Ag2 S Semiconductor.

Xue-Feng Zhao, Shi-Qi Yang, Xiao-Hong Wen, Qi-Wei Huang, Peng-Fei Qiu, Tian-Ran Wei, Hao Zhang, Jia-Cheng Wang, David Wei Zhang, Xun Shi, Hong-Liang Lu,

Wearable touch panel, a typical flexible electronic device, can recognize and feedback the information of finger touch and movement. Excellent wearable touch panels are required to accurately and quickly monitor the signals of finger movement as well as the capacity of bearing various deformation. High-performance thermistor materials are one of ... Read more >>

Adv Mater (Advanced materials (Deerfield Beach, Fla.))
[2022, :e2107479]

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Observation of Three-Dimensional Biexcitons in Pristine-Quality CH3 NH3 PbBr3 Single Crystals.

Hongsun Ryu, Jeehong Park, Seo Hyun Nam, Joon Woo Park, Kitae Kim, Yeonjin Yi, Joon I Jang,

Halide perovskites (HPs) are fascinating materials whose optoelectronic properties are arguably excitonic. In the HP family, biexcitons are known to exist only in low dimensions where exciton-exciton binding is strongly enhanced by quantum and dielectric confinements. In this paper, however, we show that they indeed do exist in three-dimensional (3D) ... Read more >>

Adv Mater (Advanced materials (Deerfield Beach, Fla.))
[2022, :e2107882]

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Jammed Micro-Flake Hydrogel for 4D Living Cell Bioprinting.

Aixiang Ding, Oju Jeon, David Cleveland, Kaelyn Gasvoda, Derrick Wells, Sang Jin Lee, Eben Alsberg,

Four-dimensional (4D) bioprinting is promising to build cell-laden constructs (bioconstructs) with complex geometries and functions for tissue/organ regeneration applications. The development of hydrogel-based 4D bioinks, especially those allowing living cell printing, with easy preparation, defined composition, and controlled physical properties is critically important for 4D bioprinting. Here, a single-component jammed ... Read more >>

Adv Mater (Advanced materials (Deerfield Beach, Fla.))
[2022, :e2109394]

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Highly Efficient Cellular Acoustic Absorber of Graphene Ultrathin Drums.

Kai Pang, Xiaoting Liu, Jintao Pang, Akram Samy, Jin Xie, Yingjun Liu, Li Peng, Zhen Xu, Chao Gao,

Atomically thin two-dimensional graphene sheet exhibits unparalleled in-plane stiffness and large out-of-plane elasticity, thereby provides strong mechanical resonance for nanomechanical devices. The exceptional resonance behavior of ultrathin graphene promises to the fabrication of superior acoustic absorption materials, however, remains unfulfilled for the lack of applicable form and assembly methods. Here, ... Read more >>

Adv Mater (Advanced materials (Deerfield Beach, Fla.))
[2022, :e2103740]

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Asymmetric Chemical Functionalization of Top-Contact Electrodes: Tuning the Charge Injection for High Performance MoS2 Field-Effect Transistors and Schottky Diodes.

Bin Han, Yuda Zhao, Chun Ma, Can Wang, Xinzi Tian, Ye Wang, Wenping Hu, Paolo Samorì,

The fabrication of high-performance (opto-)electronic devices based on ultrathin two-dimensional channel materials requires the optimization of the charge injection at the electrode - semiconductor interface. While the chemical functionalization with chemisorbed self-assembled monolayers has been extensively exploited to adjust the work function of metallic electrodes in bottom-contact devices, such a ... Read more >>

Adv Mater (Advanced materials (Deerfield Beach, Fla.))
[2022, :e2109445]

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Magnetic Skyrmions in a Thickness Tunable 2D Ferromagnet from a Defect Driven Dzyaloshinskii-Moriya Interaction.

Anirban Chakraborty, Abhay K Srivastava, Ankit K Sharma, Ajesh K Gopi, Katayoon Mohseni, Arthur Ernst, Hakan Deniz, Binoy Krishna Hazra, Souvik Das, Paolo Sessi, Ilya Kostanovskiy, Tianping Ma, Holger L Meyerheim, Stuart S P Parkin,

There is considerable interest in van der Waals (vdW) materials as potential hosts for chiral skyrmionic spin textures. Of particular interest is the ferromagnetic, metallic compound Fe<sub>3</sub> GeTe<sub>2</sub> (FGT), which has a comparatively high Curie temperature (150-220 K). Several recent studies have reported the observation of chiral Néel skyrmions in ... Read more >>

Adv Mater (Advanced materials (Deerfield Beach, Fla.))
[2022, :e2108637]

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Application of Nanostructured TiO2 in UV Photodetectors: A Review.

Ziliang Li, Ziqing Li, Chaolei Zuo, Xiaosheng Fang,

As a wide bandgap inorganic semiconductor material, the titanium dioxide (TiO2 ) which possesses 3 crystal polymorphs (i.e., rutile, anatase and brookite), has gained tremendous attention as a cutting-edge material for the application in environment and energy field. Based on the strong attractiveness from its advantages such as high stability, excellent ... Read more >>

Adv Mater (Advanced materials (Deerfield Beach, Fla.))
[2022, :e2109083]

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Biomimetic Nanoerythrosome-Coated Aptamer-DNA Tetrahedron/Maytansine Conjugates: pH-Responsive and Targeted Cytotoxicity for HER2-positive Breast Cancer.

Wenjuan Ma, Yuting Yang, Jianwei Zhu, Weiqiang Jia, Tao Zhang, Zhiqiang Liu, Xingyu Chen, Yunfeng Lin,

DNA materials have emerged as potential nanocarriers for targeted cancer therapy with superior biological applications to precisely deliver cargo with specific purpose. However, many DNA carriers have constrained ability to carry sufficient dose of drugs, and their short half-life and low bioavailability due to the interception by the reticuloendothelial system ... Read more >>

Adv Mater (Advanced materials (Deerfield Beach, Fla.))
[2022, :e2109609]

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