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Journal ACS Appl Mater Interfaces

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Multifunctional Soft Robotic Finger Based on a Nanoscale Flexible Temperature-Pressure Tactile Sensor for Material Recognition.

Wentuo Yang, Mengying Xie, Xiaoshuang Zhang, Xueyou Sun, Cheng Zhou, Ye Chang, Hainan Zhang, Xuexin Duan,

Robotic hands with tactile perception can perform more advanced and safer operations, such as material recognition. Nanowires with high sensitivity, fast response, and low power consumption are suitable for multifunctional flexible tactile sensors to provide the tactile perception of robotic hands. In this work, we designed a multifunctional soft robotic ... Read more >>

ACS Appl Mater Interfaces (ACS applied materials & interfaces)
[2021, 13(46):55756-55765]

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High-Performance Oxide-Based p-n Heterojunctions Integrating p-SnOx and n-InGaZnO.

Dong Hun Lee, Honghwi Park, Michael Clevenger, Hyeonghun Kim, Chung Soo Kim, Mingyuan Liu, Giyong Kim, Han Wook Song, Kwangsoo No, Sung Yeol Kim, Dong-Kyun Ko, Anne Lucietto, Hongsik Park, Sunghwan Lee,

The fabrication of oxide-based p-n heterojunctions that exhibit high rectification performance has been difficult to realize using standard manufacturing techniques that feature mild vacuum requirements, low thermal budget processing, and scalability. Critical bottlenecks in the fabrication of these heterojunctions include the narrow processing window of p-type oxides and the charge-blocking ... Read more >>

ACS Appl Mater Interfaces (ACS applied materials & interfaces)
[2021, 13(46):55676-55686]

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Unraveling a Graphene Exfoliation Technique Analogy in the Making of Ultrathin Nickel-Iron [email protected] Foam to Promote the OER.

Zubair Ahmed, Krishankant, Ritu Rai, Rajinder Kumar, Takahiro Maruyama, Chandan Bera, Vivek Bagchi,

One of the major objectives of using the improved Hummers' method was to exfoliate the graphene layers by oxidizing and thereafter reducing them to obtain highly conductive reduced graphene layers, which can be used in the construction of electronic devices or as a part of catalyst composites in energy conversion ... Read more >>

ACS Appl Mater Interfaces (ACS applied materials & interfaces)
[2021, 13(46):55281-55291]

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Insights on the Properties of the O-Doped Argyrodite Sulfide Solid Electrolytes (Li6PS5-xClOx,x=0-1).

Zhen Sun, Yanqing Lai, Na Lv, Yaqi Hu, Bingqin Li, Liangxing Jiang, Jiong Wang, Shuo Yin, Kui Li, Fangyang Liu,

Argyrodite sulfide solid electrolytes, such as Li6PS5Cl (LPSC), have received much attention due to their high ionic conductivity (>1 mS cm-1) and success in all-solid-state batteries (long cycle performance, high energy density, etc.). Numerous efforts are spent on modifying the properties of the electrolyte itself. Here, we combine first-principles calculations ... Read more >>

ACS Appl Mater Interfaces (ACS applied materials & interfaces)
[2021, 13(46):54924-54935]

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Rational Design on Controllable Cation Injection with Improved Conductive-Bridge Random Access Memory by Glancing Angle Deposition Technology toward Neuromorphic Application.

Yu-Chuan Shih, Ying-Chun Shen, Yen-Kai Cheng, Mayur Chaudhary, Tzu-Yi Yang, Yi-Jen Yu, Yu-Lun Chueh,

A conductive-bridge random access memory (CBRAM) has been considered a promising candidate for the next-generation nonvolatile memory technology because of its excellent performance, for which the resistive switching behavior depends on the formation/dissolution of conducting filaments in an electrolyte layer originated by the cation injection from the active electrode with ... Read more >>

ACS Appl Mater Interfaces (ACS applied materials & interfaces)
[2021, 13(46):55470-55480]

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Activation of Mechanophores in a Thermoset Matrix by Instrumented Scratch.

Chelsea S Davis, Mitchell L Rencheck, Jeremiah W Woodcock, Ryan Beams, Muzhou Wang, Stephan Stranick, Aaron M Forster, Jeffrey W Gilman,

Scratches in polymer coatings and barrier layers negatively impact optical properties (haze, light transmission, etc.), initiate routes of degradation or corrosion (moisture permeability), and nucleate delamination of the coating. Detecting scratches in coatings on advanced materials systems is an important component of structural health monitoring but can be difficult if ... Read more >>

ACS Appl Mater Interfaces (ACS applied materials & interfaces)
[2021, 13(46):55498-55506]

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Scalable Characterization of 2D Gallium-Intercalated Epitaxial Graphene.

Hesham El-Sherif, Natalie Briggs, Brian Bersch, Minghao Pan, Mahdi Hamidinejad, Siavash Rajabpour, Tobin Filleter, Ki Wook Kim, Joshua Robinson, Nabil D Bassim,

Scalable synthesis of two-dimensional gallium (2D-Ga) covered by graphene layers was recently realized through confinement heteroepitaxy using silicon carbide substrates. However, the thickness, uniformity, and area coverage of the 2D-Ga heterostructures have not previously been studied with high-spatial resolution techniques. In this work, we resolve and measure the 2D-Ga heterostructure ... Read more >>

ACS Appl Mater Interfaces (ACS applied materials & interfaces)
[2021, 13(46):55428-55439]

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Ultra-High-Capacity and Dendrite-Free Zinc-Sulfur Conversion Batteries Based on a Low-Cost Deep Eutectic Solvent.

Mangwei Cui, Jinbo Fei, Funian Mo, Hao Lei, Yan Huang,

Traditional cathodes for aqueous Zn-ion batteries are afflicted by a limited specific capacity and fearful Zn dendrites. Herein, these troubles are disposed of with a conversion-type Zn-S battery and low-cost deep eutectic solvent (DES). By utilizing the optimized electrolyte, the symmetrical Zn battery can stably cycle over 3920 h, which ... Read more >>

ACS Appl Mater Interfaces (ACS applied materials & interfaces)
[2021, 13(46):54981-54989]

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Sunflower-Stalk-Based Solar-Driven Evaporator with a Confined 2D Water Channel and an Enclosed Thermal-Insulating Cellular Structure for Stable and Efficient Steam Generation.

Fangqingxin Liu, Linmin Xia, Lingyan Zhang, Fei Guo, Xuexia Zhang, Yan Yu, Rilong Yang,

Given the worsening freshwater scarcity around the world, the interfacial solar-driven steam generation for seawater desalination and wastewater treatment has attracted wide attention due to its rich energy resources, convenience, and environmental friendliness. However, challenges still remain for developing high-efficiency interfacial solar-driven steam generation devices from low-cost, readily available, and ... Read more >>

ACS Appl Mater Interfaces (ACS applied materials & interfaces)
[2021, 13(46):55299-55306]

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Reaction Mechanism and Strategy for Optimizing the Hydrogen Evolution Reaction on Single-Layer 1T' WSe2 and WTe2 Based on Grand Canonical Potential Kinetics.

Jie Song, Soonho Kwon, Md Delowar Hossain, Sheng Chen, Zhenyu Li, William A Goddard,

Transition-metal dichalcogenides (TMDs) in the 1T' phase are known high-performance catalysts for hydrogen evolution reaction (HER). Many experimental and some theoretical studies report that vacant sites play an important role in the HER on the basal plane. To provide benchmark calculations for comparison directly with future experiments on TMDs to ... Read more >>

ACS Appl Mater Interfaces (ACS applied materials & interfaces)
[2021, 13(46):55611-55620]

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High-Performance Flexible InAs Thin-Film Photodetector Arrays with Heteroepitaxial Growth Using an Abruptly Graded InxAl1-xAs Buffer.

Seungwan Woo, Geunhwan Ryu, Soo Seok Kang, Tae Soo Kim, Namgi Hong, Jae-Hoon Han, Rafael Jumar Chu, In-Hwan Lee, Daehwan Jung, Won Jun Choi,

Current infrared thermal image sensors are mainly based on planar firm substrates, but the rigid form factor appears to restrain the versatility of their applications. For wearable health monitoring and implanted biomedical sensing, transfer of active device layers onto a flexible substrate is required while controlling the high-quality crystalline interface. ... Read more >>

ACS Appl Mater Interfaces (ACS applied materials & interfaces)
[2021, 13(46):55648-55655]

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Interconnected MoS2 on 2D Graphdiyne for Reversible Sodium Storage.

Jing Xu, Qing Liu, Zhong Dong, Lina Wang, Xingchen Xie, Yong Jiang, Zhengnan Wei, Yongping Gao, Yu Zhang, Kejing Huang,

In this study, graphdiyne (GDY) was first reported as a substrate material for sodium-ion batteries (SIBs). The creative hybridization of GDY and molybdenum disulfide (MoS2) endows the composite with unique heterostructural and morphological advantages that boost the charge transport rate and enhance the battery discharge properties. Electrochemical results indicated that ... Read more >>

ACS Appl Mater Interfaces (ACS applied materials & interfaces)
[2021, 13(46):54974-54980]

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Optimum Hydrogen Injection in Phosphorus-Doped Polysilicon Passivating Contacts.

Di Kang, Hang Cheong Sio, Josua Stuckelberger, Rong Liu, Di Yan, Xinyu Zhang, Daniel Macdonald,

It has previously been shown that ex situ phosphorus-doped polycrystalline silicon on silicon oxide (poly-Si/SiOx) passivating contacts can suffer a pronounced surface passivation degradation when subjected to a firing treatment at 800 °C or above. The degradation behavior depends strongly on the processing conditions, such as the dielectric coating layers ... Read more >>

ACS Appl Mater Interfaces (ACS applied materials & interfaces)
[2021, 13(46):55164-55171]

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Differentiated Oxygen Evolution Behavior in MOF-Derived Oxide Nanomaterials Induced by Phase Transition.

Li Zhong, Xian Wang, Yuanyuan Guo, Junyang Ding, Qi Huang, Ting-Ting Li, Yue Hu, Jinjie Qian, Shaoming Huang,

Oxygen evolution reaction (OER) on the anode has become one of the most widely studied electrochemical processes, which poses an important role in several energy generation technologies. In this work, we have designed and synthesized a series of metal-organic framework (MOF)-derived oxides pyrolyzed at different temperatures for efficient water oxidation ... Read more >>

ACS Appl Mater Interfaces (ACS applied materials & interfaces)
[2021, 13(46):55454-55462]

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Carbon-Free Crystal-like Fe1-xS as an Anode for Potassium-Ion Batteries.

Yuhan Wu, Rui Xu, Zhijie Wang, Xiaorui Hao, Chenglin Zhang, Huaping Zhao, Wei Li, Shouzhi Wang, Yulian Dong, Zhitao Huang, Yong Lei,

Potassium-ion batteries (PIBs) as a new electrochemical energy storage system have been considered as a desirable candidate in the post-lithium-ion battery era. Nevertheless, the study on this realm is in its infancy; it is urgent to develop electrode materials with high electrochemical performance and low cost. Iron sulfides as anode ... Read more >>

ACS Appl Mater Interfaces (ACS applied materials & interfaces)
[2021, 13(46):55218-55226]

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3D Carbon-Based Porous Anode with a Pore-Size Gradient for High-Performance Lithium Metal Batteries.

Hyeon-Jae Noh, Min-Ho Lee, Byung Gon Kim, Jun-Ho Park, Sang-Min Lee, Jeong-Hee Choi,

Three-dimensional (3D) hosts have been identified as the most promising anode design for lithium metal batteries (LMBs). This has been previously demonstrated to be extremely effective at inhibiting the dendrite growth by reducing the local current densities, resulting in stable cycle performances. However, due to the complex synthetic procedures and ... Read more >>

ACS Appl Mater Interfaces (ACS applied materials & interfaces)
[2021, 13(46):55227-55234]

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Ultrathin Superhydrophobic Flexible Tactile Sensors for Normal and Shear Force Discrimination.

Mengpei Zhang, Xiping Gao, Chang Lu, Dahu Yao, Lanlan Wu, Dongxue Li, Hanqing Fang, Shiwei A, Yafei Sun,

Flexible tactile sensors, with the ability to sense and even discriminate between different mechanical stimuli, can enable real-time and precise monitoring of dexterous and complex robotic motions. However, making them ultrathin and superhydrophobic for practical applications is still a great challenge. Here, superhydrophobic flexible tactile sensors with hierarchical micro- and ... Read more >>

ACS Appl Mater Interfaces (ACS applied materials & interfaces)
[2021, :]

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Wetting Behavior of Surface Nanodroplets Regulated by Periodic Nanostructured Surfaces.

Limin Zhou, Shumin Yang, Nannan Quan, Zhanli Geng, Shuo Wang, Binyu Zhao, Xingya Wang, Yaming Dong, Renzhong Tai, Jun Hu, Lijuan Zhang,

Surfaces with nanostructure patterning are broadly encountered in nature, and they play a significant role in regulating various phenomena such as phase transition at the liquid/solid interface. Here, we designed two kinds of template substrates with periodic nanostructure patterns [i.e., nanotrench (NT) and nanopore (NP)]. Surface nanodroplets produced on these ... Read more >>

ACS Appl Mater Interfaces (ACS applied materials & interfaces)
[2021, :]

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Organic/Inorganic Hybrid Thin-Film Encapsulation Using Inkjet Printing and PEALD for Industrial Large-Area Process Suitability and Flexible OLED Application.

Byoung-Hwa Kwon, Chul Woong Joo, Hyunsu Cho, Chan-Mo Kang, Jong-Heon Yang, Jin-Wook Shin, Gi Heon Kim, Sukyung Choi, Sooji Nam, Kukjoo Kim, Chun-Won Byun, Nam Sung Cho, Sujung Kim,

We present herein the first report of organic/inorganic hybrid thin-film encapsulation (TFE) developed as an encapsulation process for mass production in the display industry. The proposed method was applied to fabricate a top-emitting organic light-emitting device (TEOLED). The organic/inorganic hybrid TFE has a 1.5 dyad structure and was fabricated using ... Read more >>

ACS Appl Mater Interfaces (ACS applied materials & interfaces)
[2021, :]

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Screening of Adsorbent/Catalyst Composite Monoliths for Carbon Capture-Utilization and Ethylene Production.

Shane Lawson, Khaled Baamran, Kyle Newport, Fateme Rezaei, Ali Rownaghi,

Combining CO<sub>2</sub> adsorption and utilization in oxidative dehydrogenation of ethane (ODHE) into a single bed is an exciting way of converting a harmful greenhouse gas into marketable commodity chemicals while reducing energy requirements from two-bed processes. However, novel materials should be developed for this purpose because most adsorbents are incapable ... Read more >>

ACS Appl Mater Interfaces (ACS applied materials & interfaces)
[2021, :]

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Mo/P Dual-Doped Co/Oxygen-Deficient Co3O4 Core-Shell Nanorods Supported on Ni Foam for Electrochemical Overall Water Splitting.

Yawen Hao, Gaohui Du, Yi Fan, Lina Jia, Di Han, Wenqi Zhao, Qingmei Su, Shukai Ding, Bingshe Xu,

The exploration for low-cost bifunctional materials for highly efficient overall water splitting has drawn profound research attention. Here, we present a facile preparation of Mo-P dual-doped Co/oxygen-deficient Co<sub>3</sub>O<sub>4</sub> core-shell nanorods as a highly efficient electrocatalyst. In this strategy, oxygen vacancies are first generated in Co<sub>3</sub>O<sub>4</sub> nanorods by lithium reduction at ... Read more >>

ACS Appl Mater Interfaces (ACS applied materials & interfaces)
[2021, :]

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PIM-1/Holey Graphene Oxide Mixed Matrix Membranes for Gas Separation: Unveiling the Role of Holes.

Jose Miguel Luque-Alled, Marzieh Tamaddondar, Andrew B Foster, Peter M Budd, Patricia Gorgojo,

PIM-1/holey graphene oxide (GO) mixed matrix membranes (MMMs) have been prepared and their gas separation performance for CO<sub>2</sub>/CH<sub>4</sub> mixtures assessed. Nanopores have been created in the basal plane of gas-impermeable GO by chemical etching reactions, and the resulting holey flakes have been further chemically functionalized, either with octadecylamine (ODA) or ... Read more >>

ACS Appl Mater Interfaces (ACS applied materials & interfaces)
[2021, :]

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Multifunctional Mechanical Sensing Electronic Device Based on Triboelectric Anisotropic Crumpled Nanofibrous Mats.

Yinben Guo, Zixi Chen, Weifeng Yang, Kerui Li, Dongye Yang, Qinghong Zhang, Hongzhi Wang,

Integrating multiple mechanical sensing capabilities in one device is highly desired to mimic the amazing functions of human skin, and it demonstrates promising applications in the human-machine interface and wearable robotic exoskeletons. Yet, challenges remain in how to couple the multisensations using as few modules as possible to increase the ... Read more >>

ACS Appl Mater Interfaces (ACS applied materials & interfaces)
[2021, 13(46):55481-55488]

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General One-Pot Method for Preparing Highly Water-Soluble and Biocompatible Photoinitiators for Digital Light Processing-Based 3D Printing of Hydrogels.

Hui Wang, Biao Zhang, Jianhong Zhang, Xiangnan He, Fukang Liu, Jingjing Cui, Zhe Lu, Guang Hu, Jun Yang, Zhe Zhou, Runze Wang, Xingyu Hou, Luankexin Ma, Panyu Ren, Qi Ge, Peng Li, Wei Huang,

We report a facile but general method to prepare highly water-soluble and biocompatible photoinitiators for digital light processing (DLP)-based 3D printing of high-resolution hydrogel structures. Through a simple and straightforward one-pot procedure, we can synthesize a metal-phenyl(2,4,6-trimethylbenzoyl)phosphinates (M-TMPP)-based photoinitiator with excellent water solubility (up to ∼50 g/L), which is much ... Read more >>

ACS Appl Mater Interfaces (ACS applied materials & interfaces)
[2021, 13(46):55507-55516]

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Dual Porous 3D Zinc Anodes toward Dendrite-Free and Long Cycle Life Zinc-Ion Batteries.

Kai Chen, Huinan Guo, Weiqin Li, Yijing Wang,

Rechargeable aqueous zinc-ion batteries (ZIBs) have been proven to be an alternative energy storage system because of their high safety, low cost, and eco-friendliness. However, the poor stability of metallic Zn anodes suffering from uncontrolled dendrite formation and electrochemical corrosion has brought troublesome hindrances for their practical application. In this ... Read more >>

ACS Appl Mater Interfaces (ACS applied materials & interfaces)
[2021, 13(46):54990-54996]

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