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Fracture toughness of a metal-organic framework glass.

Theany To, Søren S Sørensen, Malwina Stepniewska, Ang Qiao, Lars R Jensen, Mathieu Bauchy, Yuanzheng Yue, Morten M Smedskjaer,

Metal-organic framework glasses feature unique thermal, structural, and chemical properties compared to traditional metallic, organic, and oxide glasses. So far, there is a lack of knowledge of their mechanical properties, especially toughness and strength, owing to the challenge in preparing large bulk glass samples for mechanical testing. However, a recently ... Read more >>

Nat Commun (Nature communications)
[2020, 11(1):2593]

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Observation of indentation-induced shear bands in a metal-organic framework glass.

Malwina Stepniewska, Kacper Januchta, Chao Zhou, Ang Qiao, Morten M Smedskjaer, Yuanzheng Yue,

Metal-organic framework (MOF) glasses are a newly emerged family of melt-quenched glasses. Recently, several intriguing features, such as ultrahigh glass-forming ability and low liquid fragility, have been discovered in a number of zeolitic imidazolate frameworks (ZIFs) that are a subset of MOFs. However, the fracture behavior of ZIF glasses has ... Read more >>

Proc. Natl. Acad. Sci. U.S.A. (Proceedings of the National Academy of Sciences of the United States of America)
[2020, 117(19):10149-10154]

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Structural evolution in a melt-quenched zeolitic imidazolate framework glass during heat-treatment.

Jiayan Zhang, Louis Longley, Hao Liu, Christopher W Ashling, Philip A Chater, Kevin A Beyer, Karena W Chapman, Haizheng Tao, David A Keen, Thomas D Bennett, Yuanzheng Yue,

A pronounced enthalpy release occurs around 1.38Tg in the prototypical metal-organic framework glass formed from ZIF-4 [Zn(C3H3N2)2], but there is no sign for any crystallization (i.e., long-range ordering) taking place. The enthalpy release peak is attributed to pore collapse and structural densification. ... Read more >>

Chem. Commun. (Camb.) (Chemical communications (Cambridge, England))
[2019, 55(17):2521-2524]

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Metal-Organic Framework Glasses Possess Higher Thermal Conductivity than Their Crystalline Counterparts.

Søren S Sørensen, Martin B Østergaard, Malwina Stepniewska, Hicham Johra, Yuanzheng Yue, Morten M Smedskjaer,

The thermal conductivity (κ) of glasses is known to always be lower than that of their corresponding crystals due to the stronger phonon-phonon scattering in the former. However, it is unknown whether this relation holds for metal-organic frameworks. Here, we report our discovery of an inverse relation in κ between ... Read more >>

ACS Appl Mater Interfaces (ACS applied materials & interfaces)
[2020, 12(16):18893-18903]

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Ultrahigh-field 67Zn NMR reveals short-range disorder in zeolitic imidazolate framework glasses.

Rasmus S K Madsen, Ang Qiao, Jishnu Sen, Ivan Hung, Kuizhi Chen, Zhehong Gan, Sabyasachi Sen, Yuanzheng Yue,

The structure of melt-quenched zeolitic imidazole framework (ZIF) glasses can provide insights into their glass-formation mechanism. We directly detected short-range disorder in ZIF glasses using ultrahigh-field zinc-67 solid-state nuclear magnetic resonance spectroscopy. Two distinct Zn sites characteristic of the parent crystals transformed upon melting into a single tetrahedral site with ... Read more >>

Science (Science (New York, N.Y.))
[2020, 367(6485):1473-1476]

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Dissolution of Stone Wool Fibers with Phenol-urea-formaldehyde Binder in a Synthetic Lung Fluid.

Susanne H Q Barly, Denis V Okhrimenko, Mette Solvang, Yuanzheng Yue, Susan L S Stipp,

Mineral wool products, composed of stone wool fibers and organic binder, are used in many construction applications. Among all their beneficial properties, the most important requirement is safety for human health, such as when fibers are inhaled. For determining long-term toxicity, biosolubility and biopersistence studies in vitro and in vivo ... Read more >>

Chem. Res. Toxicol. (Chemical research in toxicology)
[2019, 32(12):2398-2410]

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Genome-wide investigation of WRKY transcription factors in sweet osmanthus and their potential regulation of aroma synthesis.

Wenjie Ding, Qixia Ouyang, Yuli Li, Tingting Shi, Ling Li, Xiulian Yang, Kongshu Ji, Lianggui Wang, Yuanzheng Yue,

WRKY transcription factors, one of the largest transcription factor families, play important roles in regulating the synthesis of secondary metabolites. In sweet osmanthus (Osmanthus fragrans), the monoterpenes have been demonstrated as the most important volatile compounds, and the W-box, which is the cognate binding site of WRKY transcription factors, could ... Read more >>

Tree Physiol. (Tree physiology)
[2020, 40(4):557-572]

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SSR marker development in Clerodendrum trichotomum using transcriptome sequencing.

Gongwei Chen, Yuanzheng Yue, Yajie Hua, Die Hu, Tingting Shi, Zhaojing Chang, Xiulian Yang, Lianggui Wang,

Clerodendrum trichotomum, a member of the Lamiaceae (Verbenaceae) family, is an ornamental plant widely distributed in South Asia. Previous studies have focused primarily on its growth characteristics, stress resistance, and pharmacological applications; however, molecular investigations remain limited. Considering germplasm conservation and the extensive applications of this plant, it is necessary ... Read more >>

PLoS ONE (PloS one)
[2019, 14(11):e0225451]

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Exploration of Floral Volatile Organic Compounds in Six Typical Lycoris taxa by GC-MS.

Tingting Shi, Yuanzheng Yue, Man Shi, Min Chen, Xiulian Yang, Lianggui Wang,

Lycoris, which is known as the 'Chinese tulip,' has diverse flower colors and shapes, and some species have a delicate fragrance. However, limited studies have reported the volatile organic compounds (VOCs) of Lycoris. In this study, headspace solid-phase microextraction combined with gas chromatography-mass spectrometry was used to analyze the floral ... Read more >>

Plants (Basel) (Plants (Basel, Switzerland))
[2019, 8(10):]

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Genome-Wide Identification and Characterization of JAZ Protein Family in Two Petunia Progenitors.

Shaoze Tian, Siyu Liu, Yu Wang, Kun Wang, Chaoqun Yin, Yuanzheng Yue, Huirong Hu,

Jasmonate ZIM-domain (JAZ) family proteins are the key repressors in the jasmonate signaling pathway and play crucial roles in plant development, defenses, and responses to stresses. However, our knowledge about the JAZ protein family in petunia is limited. This research respectively identified 12 and 16 JAZ proteins in two Petunia ... Read more >>

Plants (Basel) (Plants (Basel, Switzerland))
[2019, 8(7):]

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Selection of appropriate reference genes for quantitative real-time PCR in Clerodendrum trichotomum

Yajie Hua, Yuanzheng Yue, Gongwei Chen, Taotao Yan, Wenjie Ding, Tingting Shi, Die Hu, Lianggui Wang, Xiulian Yang,

Abstrsct Clerodendrum trichotomum , an important medicinal plant, has excellent salt tolerance and beautiful ornamental character. However, reliable reference genes for quantitative real-time PCR data (qRT-PCR) in C. trichotomum have not been investigated. Using our previous transcriptome data, 17 reference genes were selected in different tissues (leaves, flowers, fruits, stems, ... Read more >>

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Understanding Glass through Differential Scanning Calorimetry.

Qiuju Zheng, Yanfei Zhang, Maziar Montazerian, Ozgur Gulbiten, John C Mauro, Edgar D Zanotto, Yuanzheng Yue,

Differential scanning calorimetry (DSC) is a powerful tool to address some of the most challenging issues in glass science and technology, such as the nonequilibrium nature of the glassy state and the detailed thermodynamics and kinetics of glass-forming systems during glass transition, relaxation, rejuvenation, polyamorphic transition, and crystallization. The utility ... Read more >>

Chem. Rev. (Chemical reviews)
[2019, 119(13):7848-7939]

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Erratum: Author Correction: The chromosome-level quality genome provides insights into the evolution of the biosynthesis genes for aroma compounds of Osmanthus fragrans.

Xiulian Yang, Yuanzheng Yue, Haiyan Li, Wenjie Ding, Gongwei Chen, Tingting Shi, Junhao Chen, Min S Park, Fei Chen, Lianggui Wang,

[This corrects the article DOI: 10.1038/s41438-018-0108-0.]. ... Read more >>

Hortic Res (Horticulture research)
[2019, 6:62]

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Integrating Transcriptomic and GC-MS Metabolomic Analysis to Characterize Color and Aroma Formation during Tepal Development in Lycoris longituba.

Yuanzheng Yue, Jiawei Liu, Tingting Shi, Min Chen, Ya Li, Juhua Du, Haiyan Jiang, Xiulian Yang, Huirong Hu, Lianggui Wang,

Lycoris longituba, belonging to the Amaryllidaceae family, is a perennial bulb bearing flowers with diverse colors and fragrance. Selection of cultivars with excellent colored and scented flowers has always been the breeding aim for ornamental plants. However, the molecular mechanisms underlying color fading and aroma production during flower expansion in ... Read more >>

Plants (Basel) (Plants (Basel, Switzerland))
[2019, 8(3):]

Cited: 4 times

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Optical properties of a melt-quenched metal-organic framework glass.

Ang Qiao, Haizheng Tao, Michael P Carson, Scott W Aldrich, Lynn M Thirion, Thomas D Bennett, John C Mauro, Yuanzheng Yue,

Metal-organic framework (MOF) glasses are characterized by the possession of both inorganic and organic components, linked in a continuous network structure by coordination bonds. To the best of our knowledge, the optical properties of MOF glasses have not been reported until now. In this work, we prepared a transparent bubble-free ... Read more >>

Opt Lett (Optics letters)
[2019, 44(7):1623-1625]

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Anomalous Cracking in a Metal-Organic Framework Glass

Malwina Stepniewska, Kacper Januchta, Chao Zhou, Ang Qiao, Morten Smedskjaer, Yuanzheng Yue,

<p>Metal-organic framework (MOF) glasses is a newly discovered family of melt-quenched glasses. Recently, several intriguing features (e.g., ultrahigh glass forming ability and low liquid fragility) have been discovered in the glasses obtained from zeolitic imidazolate frameworks (ZIFs) that are a subset of MOFs. However, the fracture behavior of ZIF glasses ... Read more >>

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Discovery of Superbroad Mid-Infrared Luminescent Metal-Organic Framework Glass

Mohamed. Ali, Jinjun Ren, Xiaofeng Liu, Youjie Hua, Yuanzheng Yue, Qiu Jianrong,

<p>Metal-organic framework (MOF) glasses are a newly discovered family of melt-quenched glasses. However, so far it is not known whether these glasses exhibit photonic functionalities. Here, we show the discovery of the luminescent behavior of a MOF glass, i.e., the cobalt doped zeolitic imidazolate frameworks-62 (ZIF-62) glass (Zn<sub>1-<i>x</i></sub> Co<i><sub>x</sub></i> (Im)<sub>1.9</sub> ... Read more >>

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The chromosome-level quality genome provides insights into the evolution of the biosynthesis genes for aroma compounds of Osmanthus fragrans.

Xiulian Yang, Yuanzheng Yue, Haiyan Li, Wenjie Ding, Gongwei Chen, Tingting Shi, Junhao Chen, Min S Park, Fei Chen, Lianggui Wang,

Sweet osmanthus (Osmanthus fragrans) is a very popular ornamental tree species throughout Southeast Asia and USA particularly for its extremely fragrant aroma. We constructed a chromosome-level reference genome of O. fragrans to assist in studies of the evolution, genetic diversity, and molecular mechanism of aroma development. A total of over ... Read more >>

Hortic Res (Horticulture research)
[2018, 5:72]

Cited: 4 times

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Cloning and expression analysis of three critical triterpenoid pathway genes in Osmanthus fragrans

Xiulian Yang, Wenjie Ding, Yuanzheng Yue, Chen Xu, Xi Wang, Lianggui Wang,

Osmanthus fragrans is an important ornamental tree and has been widely planted in China because of its pleasant aroma, which is mainly due to terpenes. The monoterpenoid and sesquiterpenoid metabolic pathways of sweet osmanthus have been well studied. However, these studies were mainly focused on volatile small molecule compounds. The ... Read more >>

(Electronic Journal of Biotechnology.)
[2018, 36:1-8]

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Publisher Correction: Liquid phase blending of metal-organic frameworks.

Louis Longley, Sean M Collins, Chao Zhou, Glen J Smales, Sarah E Norman, Nick J Brownbill, Christopher W Ashling, Philip A Chater, Robert Tovey, Carola-Bibiane Schönlieb, Thomas F Headen, Nicholas J Terrill, Yuanzheng Yue, Andrew J Smith, Frédéric Blanc, David A Keen, Paul A Midgley, Thomas D Bennett,

The original version of this Article contained an error in Figure 1b, where the blue '(ZIF-4-Zn)0.5 (ZIF-62)0.5 blend' data curve was omitted from the enthalpy response plot. This has now been corrected in both the PDF and HTML versions of the Article. ... Read more >>

Nat Commun (Nature communications)
[2018, 9(1):4402]

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Thermodynamic features and enthalpy relaxation in a metal-organic framework glass.

Chao Zhou, Malwina Stepniewska, Louis Longley, Christopher W Ashling, Philip A Chater, David A Keen, Thomas D Bennett, Yuanzheng Yue,

In this work, we explore the thermodynamic evolution in a melt-quenched metal-organic framework glass, formed from ZIF-62 upon heating to the melting point (Tm), and subsequent enthalpy relaxation. The temperature dependence of the difference in Gibbs free energy between the liquid and crystal states of ZIF-62 in the temperature range ... Read more >>

Phys Chem Chem Phys (Physical chemistry chemical physics : PCCP)
[2018, 20(27):18291-18296]

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Nano-phase separation and structural ordering in silica-rich mixed network former glasses.

Hao Liu, Randall E Youngman, Saurabh Kapoor, Lars R Jensen, Morten M Smedskjaer, Yuanzheng Yue,

We investigate the structure, phase separation, glass transition, and crystallization in a mixed network former glass series, i.e., B2O3-Al2O3-SiO2-P2O5 glasses with varying SiO2/B2O3 molar ratio. All the studied glasses exhibit two separate glassy phases: droplet phase (G1) with the size of 50-100 nm and matrix phase (G2), corresponding to a ... Read more >>

Phys Chem Chem Phys (Physical chemistry chemical physics : PCCP)
[2018, 20(23):15707-15717]

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Transcriptomic and GC-MS Metabolomic Analyses Reveal the Sink Strength Changes during Petunia Anther Development.

Yuanzheng Yue, Shaoze Tian, Yu Wang, Hui Ma, Siyu Liu, Yuqiao Wang, Huirong Hu,

Petunia, which has been prevalently cultivated in landscaping, is a dicotyledonous herbaceous flower of high ornamental value. Annually, there is a massive worldwide market demand for petunia seeds. The normal development of anther is the necessary prerequisite for the plants to generate seeds. However, the knowledge of petunia anther development ... Read more >>

Int J Mol Sci (International journal of molecular sciences)
[2018, 19(4):]

Cited: 4 times

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A metal-organic framework with ultrahigh glass-forming ability.

Ang Qiao, Thomas D Bennett, Haizheng Tao, Andraž Krajnc, Gregor Mali, Cara M Doherty, Aaron W Thornton, John C Mauro, G Neville Greaves, Yuanzheng Yue,

Glass-forming ability (GFA) is the ability of a liquid to avoid crystallization during cooling. Metal-organic frameworks (MOFs) are a new class of glass formers (1-3), with hitherto unknown dynamic and thermodynamic properties. We report the discovery of a new series of tetrahedral glass systems, zeolitic imidazolate framework-62 (ZIF-62) [Zn(Im2-x bIm ... Read more >>

Sci Adv (Science advances)
[2018, 4(3):eaao6827]

Cited: 5 times

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Multi-nanolayered VO2/Sapphire Thin Film via Spinodal Decomposition.

Guangyao Sun, Xun Cao, Yuanzheng Yue, Xiang Gao, Shiwei Long, Ning Li, Rong Li, Hongjie Luo, Ping Jin,

Coating of VO2-based thin film has been extensively studied for fabricating energy-saving smart windows. One of the most efficient ways for fabricating high performance films is to create multi-nanolayered structure. However, it has been highly challenge to make such layers in the VO2-based films using conventional methods. In this work, ... Read more >>

Sci Rep (Scientific reports)
[2018, 8(1):5342]

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