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Boosting the lithium-ion and sodium-ion storage performances of pyrite by regulating the energy barrier of ion transport.

Jie Wang, Jinwen Qin, Yan Jiang, Xin Wang, Minhua Cao,

Pyrite (FeS2) is a functional material of great importance for lithium/sodium ion batteries (LIBs/SIBs), but its sluggish dynamics greatly hinder its high performance. Here, we demonstrate an effective strategy of regulating the energy barrier of ion transport to significantly enhance the sluggish dynamics of FeS2 by Co doping. Compared to ... Read more >>

Nanoscale (Nanoscale)
[2020, 12(25):13781-13790]

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Twistronics in tensile strained bilayer black phosphorus.

Peng Kang, Wanting Zhang, Vincent Michaud-Rioux, Xin Wang, Jiangni Yun, Hong Guo,

In this work, by performing state-of-the-art first-principles methods combined with molecular dynamic (MD) simulation, we theoretically investigate the electronic and mechanical behaviours of small-angle twisted bilayer black phosphorus (tbBP) under uniaxial tensile deformation. Twistronics, namely the regulation of electronic properties by Moiré physics, is demonstrated as the gene - the ... Read more >>

Nanoscale (Nanoscale)
[2020, 12(24):12909-12916]

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Pressure-induced isostructural phase transition in Ti3AlC2: experimental and theoretical investigation.

Yan Li, Meiyan Ye, Ruilian Tang, Jiuhua Chen, Xin Qu, Bin Yang, Xin Wang, Huijuan Yue, Pinwen Zhu,

The structural stability of Ti3AlC2 under high pressure is important for understanding its mechanical properties. Here, we conducted a high hydrostatic pressure synchrotron X-ray diffraction experiment and no structural phase transition was observed. Like most other MAX phases, Ti3AlC2 showed an anisotropic compression behavior. Most importantly, an anomaly in c/a ... Read more >>

Phys Chem Chem Phys (Physical chemistry chemical physics : PCCP)
[2020, 22(23):13136-13142]

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Structural and physicochemical changes in almond milk during in vitro gastric digestion: impact on the delivery of protein and lipids.

Xin Wang, Aiqian Ye, Harjinder Singh,

Almond milk (about 3% protein and 7% lipids) was prepared using wet disintegration of raw almonds and then subjected to in vitro gastric digestion using an advanced dynamic digestion model (i.e., a human gastric simulator). Microstructural changes, physicochemical behavior, and protein digestion were examined; the release of lipids and protein ... Read more >>

Food Funct (Food & function)
[2020, 11(5):4314-4326]

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In situ generated nanozyme-initiated cascade reaction for amplified surface plasmon resonance sensing.

Xin Wang, Wenxin Lv, Jiahui Wu, Haiyin Li, Feng Li,

A novel nanozyme-based surface plasmon resonance (SPR) sensor was successfully developed based on the target-induced in situ generation of AuNPs and a AuNP-guided cascade reaction, with Hg2+ as the target analyte. ... Read more >>

Chem. Commun. (Camb.) (Chemical communications (Cambridge, England))
[2020, 56(33):4571-4574]

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An organoselenium-catalyzed N1- and N2-selective aza-Wacker reaction of alkenes with benzotriazoles.

Xin Wang, Qinlin Wang, Yanru Xue, Kai Sun, Lanlan Wu, Bing Zhang,

An organoselenium-catalyzed N1- and N2-selective aza-Wacker reaction of alkenes with benzotriazoles is reported, which provides easy access to N1- and N2-olefinated benzotriazole derivatives. The wide substrate scope, good functional group tolerance, and facile scale-up of this method are expected to promote its potential application in synthetic chemistry. A preliminary mechanism ... Read more >>

Chem. Commun. (Camb.) (Chemical communications (Cambridge, England))
[2020, 56(32):4436-4439]

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Hollow porous prismatic graphitic carbon nitride with nitrogen vacancies and oxygen doping: a high-performance visible light-driven catalyst for nitrogen fixation.

Ting Huang, Shugang Pan, Lingling Shi, Aiping Yu, Xin Wang, Yongsheng Fu,

Hollow porous prismatic graphitic carbon nitride with nitrogen vacancies and oxygen doping was successfully constructed using dicyandiamidine as the only raw material via a facile two-step strategy of a low-temperature hydrothermal method followed by a subsequent calcination process. The as-obtained graphitic carbon nitride showed a hollow prismatic morphology with loose ... Read more >>

Nanoscale (Nanoscale)
[2020, 12(3):1833-1841]

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Enriched environment enhances histone acetylation of NMDA receptor in the hippocampus and improves cognitive dysfunction in aged mice.

Xin Wang, Zhao-Xiang Meng, Ying-Zhu Chen, Yu-Ping Li, Hong-Yu Zhou, Man Yang, Ting-Ting Zhao, Yu-Lai Gong, Yi Wu, Tao Liu,

The mechanisms of age-associated memory impairment may be associated with glutamate receptor function and chromatin modification. To observe the effect of an enriched environment on the cognitive function of mice with age-associated memory impairment, 3-month-old C57BL/6 male mice ("young" mice) were raised in a standard environment, while 24-month-old C57BL/6 male ... Read more >>

Neural Regen Res (Neural regeneration research)
[2020, 15(12):2327-2334]

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Novel CDKs inhibitors for the treatment of solid tumour by simultaneously regulating the cell cycle and transcription control.

Xin Wang, Kaiyuan Deng, Cheng Wang, Yao Li, Tianqi Wang, Zhi Huang, Yakun Ma, Peiqing Sun, Yi Shi, Shengyong Yang, Yan Fan, Rong Xiang,

A novel series of cyclin-dependent kinases (CDKs) inhibitors, which play critical roles in the cell cycle control and regulation of cell transcription, were synthesised. A systematic study of enzymatic and cellular assays led to the identification of compound X22 with a nanomolar potency against CDK4 and CDK9 and potent antiproliferative ... Read more >>

J Enzyme Inhib Med Chem (Journal of enzyme inhibition and medicinal chemistry)
[2020, 35(1):414-423]

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Investigation on glucocorticoid receptors within platelets from adult patients with immune thrombocytopenia.

Kam Chau Yung, Cheng Wei Xu, Ze Wen Zhang, Wen Jun Yu, Qian Li, Xian Ru Xu, Ya Fei Han, Xin Jia Wang, Jun Yin,

Objective: The expression of glucocorticoid receptors within platelets from newly diagnosed Immune Thrombocytopenia (ITP) patients in the adult was investigated.Methods: GR expression in platelets from newly diagnosed ITP patients and healthy controls was measured using flow cytometry. Subsequently, platelets RNA and proteins were isolated and used for confirming the flow ... Read more >>

Hematology (Hematology (Amsterdam, Netherlands))
[2020, 25(1):37-42]

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Hierarchy of interfacial passivation in inverted perovskite solar cells.

Tun Wang, Sadeq Abbasi, Xin Wang, Yangrunqian Wang, Zhendong Cheng, Jiayuan Wang, Hong Liu, Wenzhong Shen,

The crucial hierarchy of the interfacial passivation at different positions of perovskite solar cells together with the corresponding mechanism has been studied despite the selection of passivation mediums in this work. The passivation on the upper interface could more effectively enhance the device performance with an efficiency of 19.55% compared ... Read more >>

Chem. Commun. (Camb.) (Chemical communications (Cambridge, England))
[2019, 55(99):14996-14999]

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Prussian blue-coated lanthanide-doped core/shell/shell nanocrystals for NIR-II image-guided photothermal therapy.

Xin Wang, Hui Li, Feng Li, Xiaojun Han, Guanying Chen,

Lanthanide-doped nanoparticles have long been stereotyped for optical luminescence bioimaging. However, they are known to be unable to produce therapeutic abilities. Here, we describe a lanthanide-based theranostic agent, namely, prussian blue (PB)-coated [email protected]@NaNdF4 core/shell/shell nanocrystals encapsulated in a phospholipid PEG micelle ([email protected]), which showed switched imaging and hyperthermia abilities under ... Read more >>

Nanoscale (Nanoscale)
[2019, 11(45):22079-22088]

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Rb3SbF3(NO3)3: an excellent antimony nitrate nonlinear optical material with a strong second harmonic generation response fabricated by a rational multi-component design.

Lei Wang, Fei Yang, Xiaoyu Zhao, Ling Huang, Daojiang Gao, Jian Bi, Xin Wang, Guohong Zou,

A novel antimony fluoride nitrate, Rb3SbF3(NO3)3, fabricated by a rational multi-component design, has been successfully synthesized by a rapid evaporation concentration method. This title compound crystallizes in a polar noncentrosymmetric (NCS) space group (P21) and presents a complicated three-dimensional (3D) network composed of SbO3F3, Rb-centered distorted polyhedra and π-conjugated planar ... Read more >>

Dalton Trans (Dalton transactions (Cambridge, England : 2003))
[2019, 48(40):15144-15150]

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Mechanism and origins of ligand-controlled Pd(ii)-catalyzed regiodivergent carbonylation of alkynes.

Jian-Biao Liu, Xin Zhang, Ying-Ying Tian, Xin Wang, Xun-Kun Zhu, De-Zhan Chen,

Transition-metal-catalyzed carbonylation provides a useful approach to synthesize carbonyl-containing compounds and their derivatives. Controlling the regio-, chemo-, and stereoselectivity remains a significant challenge and is the key to the success of transformation. In the present study, we explored the mechanism and origins of the ligand-controlled regiodivergent carbonylation of alkynes with ... Read more >>

Dalton Trans (Dalton transactions (Cambridge, England : 2003))
[2019, 48(40):15059-15067]

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In situ imaging of electrocatalysis in a K-O2 battery with a hollandite α-MnO2 nanowire air cathode.

Yushu Tang, Liqiang Zhang, Yongfu Tang, Xin Wang, Teng Zhang, Rui Yang, Chi Ma, Na Li, Yuening Liu, Xinxin Zhao, Xionghu Zhang, Zaifa Wang, Baiyu Guo, Yongfeng Li, Jianyu Huang,

Using α-manganese dioxide (α-MnO2) nanowires as the air electrode, a K-O2 nanobattery is assembled in an aberration corrected environmental transmission electron microscope. It is found that the α-MnO2 nanowires are reduced into Mn3O4 and MnO during discharge; meanwhile, KO2 is formed on the surface of the α-MnO2 nanowires. ... Read more >>

Chem. Commun. (Camb.) (Chemical communications (Cambridge, England))
[2019, 55(73):10880-10883]

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In situ visualization of peroxisomal peroxynitrite in the livers of mice with acute liver injury induced by carbon tetrachloride using a new two-photon fluorescent probe.

Yongqing Zhou, Ping Li, Nannan Fan, Xin Wang, Xiaoning Liu, Lijie Wu, Wen Zhang, Wei Zhang, Changle Ma, Bo Tang,

We developed a new two-photon fluorescent probe (PX-1) with high selectivity and sensitivity for detecting peroxisomal peroxynitrite. PX-1 was successfully applied to in situ imaging of peroxynitrite in the livers of mice with acute liver injury induced by carbon tetrachloride. ... Read more >>

Chem. Commun. (Camb.) (Chemical communications (Cambridge, England))
[2019, 55(47):6767-6770]

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Elevated plasma high-sensitivity C-reactive protein at admission predicts the occurrence of post-stroke fatigue at six months after ischemic stroke.

Xinjing Liu, Beng Wang, Xiao Wang, Ke Meng Tian, Xin Wang, Yan Zhang,

BACKGROUND:Post-stroke fatigue (PSF) is a common neuropsychiatric affective symptom occurring after stroke. Evidence indicates the activated inflammatory pathways are involved in modulating the stroke and fatigue. High-sensitivity C-reactive protein (hs-CRP) is one of the most sensitive indicator of inflammation. Our aim was to estimate the association between plasma hs-CRP and PSF ... Read more >>

Eur. J. Neurol. (European journal of neurology)
[2020, :]

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Clinical response to chemoradiotherapy in esophageal carcinoma is associated with survival and benefit of consolidation chemotherapy.

Zongxing Zhao, Yanan Zhang, Xin Wang, Xiaotao Geng, Liqiong Zhu, Minghuan Li,

PURPOSE:Few studies have reported the impact of the clinical response of patients with Esophageal Carcinoma to chemoradiotherapy (CRT). Our study examines the association between clinical response and pretreatment variables, survival, patterns of failure, and benefit of consolidation chemotherapy in subjects with esophageal squamous cell carcinoma (ESCC) patients receiving CRT. METHODS:Data ... Read more >>

Cancer Med (Cancer medicine)
[2020, :]

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Single atom dispersion of silicon as advanced versatile electrode material

Ze Yang, Yuwei Song, Chunfang Zhang, Jianjiang He, Xiaodong Li, Xin Wang, Ning Wang, Changshui Huang, Yuliang Li,

Abstract Silicon (Si) exhibits highest theoretical charge capacity and low discharge potential, but the associated volume expansion cannot be neglected. Here we report a single atom dispersion strategy to prepare a well distributed Si single atom based electrode material, which can effectively inhibit the volume expansion even when the storage ... Read more >>

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Glycine- and Proline-Rich Protein OsGPRP3 Regulates Grain Size and Quality in Rice.

Xin Wang, Xin Yan, Xiaoxiao Tian, Zongfei Zhang, Weiwei Wu, Junjun Shang, Jiexiu Ouyang, Wen Yao, Shaobo Li,

The grain size and shape of rice are limited by the growth of the spikelet hulls and are important selective target during domestication and breeding. In this study, we identified a glycine- and proline-rich protein (OsGPRP3), which belongs to a conserved family rarely studied. We found that OsGPRP3 was highly ... Read more >>

J. Agric. Food Chem. (Journal of agricultural and food chemistry)
[2020, :]

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Analysis of the Amplitude Changes and Baseline Drift of Respiratory Motion during Liver Stereotactic Body Radiation Therapy Based on Intra-Fraction CBCT

Lu Zeng, Xin Wang, Jidan Zhou Zhou, Pan Gong, Xuetao wang, Xiaohong Wu, Zhonghua Deng, Bin Li, Renming Zhong,

Abstract Purpose: To evaluate the amplitude changes and baseline drift of respiratory motion in liver stereotactic body radiation therapy based on intra-fraction cone beam CT (CBCT). Materials and methods : Twenty-four liver SBRT patients underwent a four-dimensional computed tomography (4D CT) scan, inter-fraction cone-beam computed tomography (CBCT), and intra-fraction CBCT ... Read more >>

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Rhodium-Catalyzed Sequential Cycloisomerization/Aldol Addition of Cyclopropene Carboxylic Acids with Isatins.

Dan Zhang, Xin Wang, Mengchu Zhang, Wenhao Hu,

A unique, rhodium-catalyzed reaction of cyclopropene carboxylic acids with isatins has been developed, which takes place through a trapping process of transient cyclic carboxylic oxonium ylides. This reaction tolerates a wide variety of cyclopropene carboxylic acids and N-protected or unprotected isatins and represents a new, direct strategy to access valuable ... Read more >>

Org. Lett. (Organic letters)
[2020, :]

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Allogeneic adipose-derived stem cells promote ischemic muscle repair by inducing M2 macrophage polarization via the HIF-1α/IL-10 pathway.

Junchao Liu, Peng Qiu, Jinbao Qin, Xiaoyu Wu, Xin Wang, Xinrui Yang, Bo Li, Wenjie Zhang, Kaichuang Ye, Zhiyou Peng, Xinwu Lu,

Adipose-derived mesenchymal stem cells (ASCs) are multipotent stromal cells that possess considerable therapeutic potential for tissue remodeling. However, their protective mechanism in critical limb ischemia (CLI) has not been fully defined. After the occlusion of blood vessels, hypoxia becomes a prominent feature of the ischemic limb. This study investigated the ... Read more >>

Stem Cells (Stem cells (Dayton, Ohio))
[2020, :]

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Perinatal listeriosis patients treated at a maternity hospital in Beijing, China, from 2013-2018

Chunyun Li, Huihui Zeng, Xin Ding, Yi Chen, Xiaowei Liu, Li Zhou, Xin Wang, Yumei Cheng, Shanshan Hu, Zheng Cao, Ruixia Liu, Chenghong Yin,

Abstract Background: Listeriosis is a rare but severe foodborne infectious disease. Perinatal listeriosis is often associated with septicemia, central nervous system (CNS) infection, and serious adverse pregnancy outcomes (miscarriage and neonate death). Here we report the characteristics and outcomes of perinatal listeriosis cases treated over 6 years at Beijing Obstetrics ... Read more >>

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Author Correction: Chromosomal translocation-derived aberrant Rab22a drives metastasis of osteosarcoma.

Dan Liao, Li Zhong, Junqiang Yin, Cuiling Zeng, Xin Wang, Xingchuan Huang, Jinna Chen, Hong Zhang, Ruhua Zhang, Xin-Yuan Guan, Xintao Shuai, Jianhua Sui, Song Gao, Wuguo Deng, Yi-Xin Zeng, Jing-Nan Shen, Jian Chen, Tiebang Kang,

An amendment to this paper has been published and can be accessed via a link at the top of the paper. ... Read more >>

Nat. Cell Biol. (Nature cell biology)
[2020, 22(7):907]

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