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Author Shuilai Qiu

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Facilely produced highly adhered, low thermal conductivity and non-combustible coatings for fire safety.

Tao Zhang, Jianchao Xi, Shuilai Qiu, Bowen Zhang, Zhangliang Luo, Weiyi Xing, Lei Song, Yuan Hu,

Fire resistant coatings have been proven as an efficient way to improve fire safety in three aspects: reducing the Heat Release Rate (HRR), delaying the ignition time and preventing heat transfer. Herein, a SiO<sub>2</sub> based polymeric composite coating with a lower thermal conductivity and brilliant fire resistance was developed. Isocyanate ... Read more >>

J Colloid Interface Sci (Journal of colloid and interface science)
[2021, 604:378-389]

Cited: 0 times

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Supramolecular wrapped sandwich like SW-Si3N4 hybrid sheets as advanced filler toward reducing fire risks and enhancing thermal conductivity of thermoplastic polyurethanes.

Liang Cheng, Jingwen Wang, Shuilai Qiu, Junling Wang, Yifan Zhou, Longfei Han, Bin Zou, Zhoumei Xu, Yuan Hu, Chao Ma,

A sandwich-like melamine/phytic acid/silicon nitride hybrid (SW-Si<sub>3</sub>N<sub>4</sub>) sheets were prepared by supramolecular wrapping as the hybrid flame retardants for thermoplastic polyurethane (TPU). The introduction of Si<sub>3</sub>N<sub>4</sub> sheets as a template could not only induce the generation of two-dimensional phytic/melamine (PAMA) capping layers, but also produce the synergistic flame-retardant effect on ... Read more >>

J Colloid Interface Sci (Journal of colloid and interface science)
[2021, 603:844-855]

Cited: 0 times

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Construction of few-layered black phosphorus/graphite-like carbon nitride binary hybrid nanostructure for reducing the fire hazards of epoxy resin.

Xiyun Ren, Bin Zou, Yifan Zhou, Zhixin Zhao, Shuilai Qiu, Lei Song,

Black phosphorus (BP) and graphite-like carbon nitride (g-C<sub>3</sub>N<sub>4</sub>) were combined to prepare BP-CN hybrid nanostructure through a simple self-assembly method assisted by ultra-sonication, and as-obtained materials were further used as fire retardants introduced into epoxy resin to fabricate EP/BP-CNx nanocomposites. It was found that the introduction of 2 wt% BP-CNx into ... Read more >>

J Colloid Interface Sci (Journal of colloid and interface science)
[2021, 586:692-707]

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Nacre-Inspired Black Phosphorus/Nanofibrillar Cellulose Composite Film with Enhanced Mechanical Properties and Superior Fire Resistance.

Shuilai Qiu, Xiyun Ren, Xia Zhou, Tao Zhang, Lei Song, Yuan Hu,

Natural nacre offers an optimized guiding principle for the assembly of lightweight and high-strength nanocomposites with excellent mechanical properties. Inspired by the "brick-and-mortar" layered structure of natural nacre, we present a cohort of bioinspired nanocomposites consisting of nanofibrillar cellulose (NFC) and few-layer hydroxyl functionalized black phosphorus (BP-OH) via a vacuum-assisted ... Read more >>

ACS Appl Mater Interfaces (ACS applied materials & interfaces)
[2020, 12(32):36639-36651]

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Construction of graphite oxide modified black phosphorus through covalent linkage: An efficient strategy for smoke toxicity and fire hazard suppression of epoxy resin.

Yifan Zhou, Fukai Chu, Shuilai Qiu, Wenwen Guo, Shenghe Zhang, Zhoumei Xu, Weizhao Hu, Yuan Hu,

The black phosphorus (BP) can be compounded with other two-dimensional materials with flame retardant effect to achieve better synergistic effect. Herein, the multifunctional BP-RGO nanohybrids was fabricated by solvothermal strategy to improve the dispersion state of BP in epoxy resin (EP) and enhance its fire safety performance, where the reduced ... Read more >>

J Hazard Mater (Journal of hazardous materials)
[2020, 399:123015]

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Combination of black phosphorus nanosheets and MCNTs via phosphoruscarbon bonds for reducing the flammability of air stable epoxy resin nanocomposites.

Bin Zou, Shuilai Qiu, Xiyun Ren, Yifan Zhou, Feng Zhou, Zhoumei Xu, Zhixin Zhao, Lei Song, Yuan Hu, Xinglong Gong,

As a rising star of two-dimensional material, black phosphorus (BP) has attracted tremendous attention in applications of photovoltaics, transistors and batteries due to its unique characteristics. Inspiring, we developed a simple strategy to fabricate BP-MCNTs as highly promising inorganic phosphorus-based flame retardant. After incorporation 2 wt% BP-MCNTs11(the mass ratio of ... Read more >>

J Hazard Mater (Journal of hazardous materials)
[2020, 383:121069]

Cited: 2 times

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Hierarchical Structure: An effective Strategy to Enhance the Mechanical Performance and Fire Safety of Unsaturated Polyester Resin.

Fukai Chu, Yanbei Hou, Longxiang Liu, Shuilai Qiu, Wei Cai, Zhoumei Xu, Lei Song, Weizhao Hu,

It is still a big challenge to prepare polymer/layered double hydroxide (LDH) composites with high performance, due to the strong agglomeration tendency of LDHs in the polymeric matrix. In this study, to avoid the agglomerated situation, the orientated LDH nanosheets were vertically grown on a ramie fabric surface, which was ... Read more >>

ACS Appl Mater Interfaces (ACS applied materials & interfaces)
[2019, 11(32):29436-29447]

Cited: 1 time

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Electrochemically Exfoliated Functionalized Black Phosphorene and Its Polyurethane Acrylate Nanocomposites: Synthesis and Applications.

Shuilai Qiu, Bin Zou, Haibo Sheng, Wenwen Guo, Junling Wang, Yuyu Zhao, Wei Wang, Richard K K Yuen, Yongchun Kan, Yuan Hu,

Owing to its mechanical performance, thermal stability, and size effects, single or few-layer black phosphorus (BP) has the potential to prepare the polymer nanocomposites as a candidate of nanoadditives, similar to graphene. The step to realize the scalable exfoliation of single or few-layer BP nanosheets is crucial to BP applications. ... Read more >>

ACS Appl Mater Interfaces (ACS applied materials & interfaces)
[2019, 11(14):13652-13664]

Cited: 1 time

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Air-Stable Polyphosphazene-Functionalized Few-Layer Black Phosphorene for Flame Retardancy of Epoxy Resins.

Shuilai Qiu, Yifan Zhou, Xia Zhou, Tao Zhang, Chenyu Wang, Richard K K Yuen, Weizhao Hu, Yuan Hu,

Similar to graphene, few-layer black phosphorus (BP) features thermal stability, mechanical properties, and characteristic dimension effects, which has potential as a new member of nanofillers for fabricating polymer nanocomposites. Herein, a cross-linked polyphosphazene-functionalized BP (BP-PZN) is developed with abundant -NH<sub>2</sub> groups via a one-pot polycondensation of 4,4'-diaminodiphenyl ether and hexachlorocyclotriphosphazene ... Read more >>

Small (Small (Weinheim an der Bergstrasse, Germany))
[2019, 15(10):e1805175]

Cited: 4 times

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Bi2Se3 decorated recyclable liquid-exfoliated MoS2 nanosheets: Towards suppress smoke emission and improve mechanical properties of epoxy resin.

Yanbei Hou, Yixin Hu, Shuilai Qiu, Longxiang Liu, Weiyi Xing, Weizhao Hu,

Bimetallic compounds have been proved superior suppression effect on smoke emission during combustion of polymers. In this work, MoS<sub>2</sub>/Bi<sub>2</sub>Se<sub>3</sub> (MB) hybrids were prepared by a facile wet chemical method and showed superior performance on smoke suppression of EP matrix during combustion. N-vinyl pyrrolidone (NVP) was employed to exfoliate molybdenum disulfide ... Read more >>

J Hazard Mater (Journal of hazardous materials)
[2019, 364:720-732]

Cited: 0 times

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Construction of Hierarchical Natural Fabric Surface Structure Based on Two-Dimensional Boron Nitride Nanosheets and Its Application for Preparing Biobased Toughened Unsaturated Polyester Resin Composites.

Fukai Chu, Dichang Zhang, Yanbei Hou, Shuilai Qiu, Junling Wang, Weizhao Hu, Lei Song,

It has been a big challenge to prepare the unsaturated polyester resin (UPR) composites with good fire safety, interfacial quality, and impact strength in an environmentally friendly way. In this study, to improve interfacial performance of fabric-reinforced UPR composites, nontoxic two-dimensional hexagonal boron nitride (h-BN) nanosheets were assembled on the ... Read more >>

ACS Appl Mater Interfaces (ACS applied materials & interfaces)
[2018, 10(46):40168-40179]

Cited: 1 time

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Construction of Bimetallic ZIF-Derived Co-Ni LDHs on the Surfaces of GO or CNTs with a Recyclable Method: Toward Reduced Toxicity of Gaseous Thermal Decomposition Products of Unsaturated Polyester Resin.

Yanbei Hou, Shuilai Qiu, Yuan Hu, Chanchal Kumar Kundu, Zhou Gui, Weizhao Hu,

This work proposed an idea of recycling in preparing Co-Ni layered double hydroxide (LDH)-derived flame retardants. A novel and feasible method was developed to synthesize CO-Ni LDH-decorated graphene oxide (GO) and carbon nanotubes (CNTs), by sacrificing bimetal zeolitic imidazolate frameworks (ZIFs). Organic ligands that departed from ZIFs were recyclable and ... Read more >>

ACS Appl Mater Interfaces (ACS applied materials & interfaces)
[2018, 10(21):18359-18371]

Cited: 1 time

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DOPO-Modified Two-Dimensional Co-Based Metal-Organic Framework: Preparation and Application for Enhancing Fire Safety of Poly(lactic acid).

Yanbei Hou, Longxiang Liu, Shuilai Qiu, Xia Zhou, Zhou Gui, Yuan Hu,

Co-based metal-organic framework (Co-MOF) nanosheets were successfully synthesized by the organic ligands with Schiff base structure. The laminated structure gives Co-MOF nanosheets a great advantage in the application in the flame retardant field. Meanwhile, -C═N- from Schiff base potentially provides active sites for further modification. In this work, 9,10-dihydro-9-oxa-10-phosphaphenanthrene-10-oxide (DOPO) ... Read more >>

ACS Appl Mater Interfaces (ACS applied materials & interfaces)
[2018, 10(9):8274-8286]

Cited: 7 times

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Melamine-containing polyphosphazene wrapped ammonium polyphosphate: A novel multifunctional organic-inorganic hybrid flame retardant.

Shuilai Qiu, Chao Ma, Xin Wang, Xia Zhou, Xiaming Feng, Richard K K Yuen, Yuan Hu,

To achieve superior fire safety epoxy resins (EP), a novel multifunctional organic-inorganic hybrid, melamine-containing polyphosphazene wrapped ammonium polyphosphate ([email protected]) with rich amino groups was prepared and used as an efficient flame retardant. Thanks to the cross-linked polyphosphazene part, [email protected] exhibited high flame retardant efficiency and smoke suppression to the EP ... Read more >>

J Hazard Mater (Journal of hazardous materials)
[2018, 344:839-848]

Cited: 10 times

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Constructing 3D Polyphosphazene [email protected] [email protected] Phosphide Ternary Nanostructures via Layer-by-Layer Method: Synthesis and Applications.

Shuilai Qiu, Yongqian Shi, Bibo Wang, Xia Zhou, Junling Wang, Chengming Wang, Chandra Sekhar Reddy Gangireddy, Richard K K Yuen, Yuan Hu,

A novel ternary nanostructure polyphosphazene nanotube (PZS)@ mesoporous silica (M-SiO<sub>2</sub>)@bimetallic phosphide (CoCuP) was facilely fabricated, using PZS as the template, where large amount of cetyltrimethylammonium bromide molecules were anchored to PZS via a similar layer-by-layer assembly strategy, and then uniform M-SiO<sub>2</sub> shells can be formed successfully by Hyeon's coating method. ... Read more >>

ACS Appl Mater Interfaces (ACS applied materials & interfaces)
[2017, 9(27):23027-23038]

Cited: 0 times

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Novel Melamine/o-Phthalaldehyde Covalent Organic Frameworks Nanosheets: Enhancement Flame Retardant and Mechanical Performances of Thermoplastic Polyurethanes.

Xiaowei Mu, Jing Zhan, Xiaming Feng, Bihe Yuan, Shuilai Qiu, Lei Song, Yuan Hu,

Covalent organic frameworks (COFs) nanosheets prepared from condensation reaction between melamine and o-phthalaldehyde are first prepared through ball milling and then incorporated into thermoplastic polyurethanes (TPU) by solution mixing. Transmission electron microscopy (TEM), X-ray diffraction (XRD), X-ray photoelectron spectroscopy (XPS), and Fourier transform infrared (FTIR) spectrometer are applied to characterize ... Read more >>

ACS Appl Mater Interfaces (ACS applied materials & interfaces)
[2017, 9(27):23017-23026]

Cited: 3 times

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Flame-retardant-wrapped polyphosphazene nanotubes: A novel strategy for enhancing the flame retardancy and smoke toxicity suppression of epoxy resins.

Shuilai Qiu, Xin Wang, Bin Yu, Xiaming Feng, Xiaowei Mu, Richard K K Yuen, Yuan Hu,

The structure of polyphosphazene nanotubes (PZS) is similar to that of carbon nanotubes (CNTs) before modification. For applications of CNTs in polymer composites, surface wrapping is an economically attractive route to achieve functionalized nanotubes. Based on this idea, functionalized polyphosphazene nanotubes ([email protected]) wrapped with a cross-linked DOPO-based flame retardant (FR) ... Read more >>

J Hazard Mater (Journal of hazardous materials)
[2017, 325:327-339]

Cited: 5 times

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A 3D Nanostructure Based on Transition-Metal Phosphide Decorated Heteroatom-Doped Mesoporous Nanospheres Interconnected with Graphene: Synthesis and Applications.

Shuilai Qiu, Weiyi Xing, Xiaowei Mu, Xiaming Feng, Chao Ma, Richard K K Yuen, Yuan Hu,

A novel three-dimensional nanostructure based on cobalt phosphide nanoparticles (Co<sub>2</sub>P NPs) and heteroatom-doped mesoporous carbon spheres interconnected with graphene (3D [email protected]<sub>2</sub>[email protected]) was facilely synthesized for the first time, and it was used for enhancing the flame retardancy and toxicity suppression of epoxy resins (EP) via a synergistic effect. Herein, the ... Read more >>

ACS Appl Mater Interfaces (ACS applied materials & interfaces)
[2016, 8(47):32528-32540]

Cited: 4 times

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Studies on Synthesis of Electrochemically Exfoliated Functionalized Graphene and Polylactic Acid/Ferric Phytate Functionalized Graphene Nanocomposites as New Fire Hazard Suppression Materials.

Xiaming Feng, Xin Wang, Wei Cai, Shuilai Qiu, Yuan Hu, Kim Meow Liew,

Practical application of functionalized graphene in polymeric nanocomposites is hampered by the lack of cost-effective and eco-friendly methods for its production. Here, we reported a facile and green electrochemical approach for preparing ferric phytate functionalized graphene (f-GNS) by simultaneously utilizing biobased phytic acid as electrolyte and modifier for the first ... Read more >>

ACS Appl Mater Interfaces (ACS applied materials & interfaces)
[2016, 8(38):25552-25562]

Cited: 2 times

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