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CpFe(CO)2 anion-catalyzed highly efficient hydrosilylation of ketones and aldehydes.

Ke Lou, Qingyang Zhou, Qi Wang, Xingchao Fan, Xiufang Xu, Chunming Cui,

K[CpFe(CO)<sub>2</sub>] and [NEt<sub>4</sub>][CpFe(CO)<sub>2</sub>] enabled highly efficient hydrosilylation of ketones and aldehydes with PhSiH<sub>3</sub> to synthesize tris- and bis(alkoxy)silanes in excellent yields depending on the substituents on the carbonyl compounds. The catalyst represents one of the most efficient and practical iron catalysts for hydrosilylation of carbonyl compounds with a TOF up ... Read more >>

Dalton Trans (Dalton transactions (Cambridge, England : 2003))
[2021, 50(32):11016-11020]

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Strain-release C-C bond cleavage enables the [2,3]-sigmatropic rearrangement of tertiary allylamines.

Rui-Han Dai, Lu Han, Qi Wang, Shi-Kai Tian,

A new strategy has been established for the [2,3]-sigmatropic rearrangement of quaternary allylammonium ylides, generated in situ from tertiary allylamines and a bicyclo[1.1.0]butane via strain-release C-C bond cleavage. A range of tertiary allylamines with an acidic α-C-H bond participated in the 1-sulfonylbicyclo[1.1.0]butane-mediated [2,3]-sigmatropic rearrangement, delivering structurally diverse N-cyclobutyl homoallylamines in ... Read more >>

Chem Commun (Camb) (Chemical communications (Cambridge, England))
[2021, 57(68):8449-8451]

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MnO2 nanosheets anchored with polypyrrole nanoparticles as a multifunctional platform for combined photothermal/photodynamic therapy of tumors.

Bei Li, Xiaodong Wang, Shasha Hong, Qi Wang, Lin Li, Omer Eltayeb, Chuan Dong, Shaomin Shuang,

Herein, [email protected]<sub>2</sub> nanocomposites were first harvested by anchoring MnO<sub>2</sub> nanosheets on polypyrrole (PPy) nanoparticles via an in situ redox reaction, then polyethylene glycol (PEG) modifier and methylene blue (MB) photosensitizer were linked through electrostatic interactions to obtain [email protected]<sub>2</sub>-PEG-MB nanoarchitectures. PPy nanoparticles ensure photothermal therapy (PTT) ability and MnO<sub>2</sub> nanosheets ameliorate ... Read more >>

Food Funct (Food & function)
[2021, 12(14):6334-6347]

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Gender-dependent reproductive toxicity of copper metal-organic frameworks and attenuation by surface modification.

Xiaotian Ji, Yousheng Mo, Haishan Li, Wanling Zhao, Aiqi Zhong, Shengqing Li, Qi Wang, Xiaopin Duan, Jisheng Xiao,

Metal-organic frameworks (MOFs) as promising materials have been widely used in drug delivery, disease diagnosis and therapy; however, their effects on the reproductive system remain unknown, which hinders their further clinical applications. Here we show that repeated subcutaneous injections of copper MOFs (HKUST-1) induce higher toxicity into the male reproductive ... Read more >>

Nanoscale (Nanoscale)
[2021, 13(15):7389-7402]

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Multifunctional l-arginine-based magnetic nanoparticles for multiple-synergistic tumor therapy.

Haiyan Yang, Fujie Jiang, Liang Zhang, Lu Wang, Yong Luo, Ningshan Li, Yu Guo, Qi Wang, Jianzhong Zou,

Tumor therapy is facing the big challenge of insufficient treatment. Here, we report high-intensity focused ultrasound (HIFU)-responsive magnetic nanoparticles based on superparamagnetic iron oxide (SPIO, Fe<sub>3</sub>O<sub>4</sub> NPs) as the shell and l-arginine (LA) as the core entrapped by poly-lactide-co-glycolide (PLGA) nanoparticles (Fe<sub>3</sub>O<sub>4</sub>@PLGA/LA NPs) for synergistic breast cancer therapy. These NPs ... Read more >>

Biomater Sci (Biomaterials science)
[2021, 9(6):2230-2243]

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Polyelectrolyte-calcium complexes as a pre-precursor induce biomimetic mineralization of collagen.

Zihuai Zhou, Leiqing Zhang, Jiachen Li, Ying Shi, Zhifang Wu, Haiyan Zheng, Zhe Wang, Weijia Zhao, Haihua Pan, Qi Wang, Xiaogang Jin, Xing Zhang, Ruikang Tang, Baiping Fu,

Polyelectrolytes such as polyaspartic acid (PAsp) are critical in biomimetic mineralization as stabilizers of amorphous calcium phosphate (ACP) precursors and as nucleation inhibitors similar to non-collagenous proteins (NCPs). Nevertheless, the application of polyelectrolyte-calcium complexes as a pre-precursor, such as PAsp-Ca complexes, in the mineralization of collagen is unexplored. Herein, we ... Read more >>

Nanoscale (Nanoscale)
[2021, 13(2):953-967]

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Prime-boost vaccination of mice and rhesus macaques with two novel adenovirus vectored COVID-19 vaccine candidates.

Shengxue Luo, Panli Zhang, Bochao Liu, Chan Yang, Chaolan Liang, Qi Wang, Ling Zhang, Xi Tang, Jinfeng Li, Shuiping Hou, Jinfeng Zeng, Yongshui Fu, Jean-Pierre Allain, Tingting Li, Yuming Zhang, Chengyao Li,

<b>ABSTRACT</b>COVID-19 vaccines are being developed urgently worldwide. Here, we constructed two adenovirus vectored COVID-19 vaccine candidates of Sad23L-nCoV-S and Ad49L-nCoV-S carrying the full-length gene of SARS-CoV-2 spike protein. The immunogenicity of two vaccines was individually evaluated in mice. Specific immune responses were observed by priming in a dose-dependent manner, and ... Read more >>

Emerg Microbes Infect (Emerging microbes & infections)
[2021, 10(1):1002-1015]

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Schizandrin A ameliorates cognitive functions via modulating microglial polarisation in Alzheimer's disease mice.

Qi Wang, Li Liu, Huibo Guan, Yanyan Zhou, Quan Li,

<h4>Context</h4>Schizandrin A (Sch A) is a major phytochemical from <i>Schisandra chinensis</i> (Turcz.) Baill. (Schisandraceae), which exerts a neuroprotective effect in Alzheimer's disease (AD).<h4>Objective</h4>To investigate the mechanism of Sch A in AD.<h4>Materials and methods</h4>AD group: APP/PS1 transgenic mice served as AD models; AD + SCH group: APP/PS1 received 2 mg/kg Sch A by intragastric ... Read more >>

Pharm Biol (Pharmaceutical biology)
[2021, 59(1):860-867]

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Potential biomarkers: differentially expressed proteins of the extrinsic coagulation pathway in plasma samples from patients with depression.

Chunyue Yu, Teli Zhang, Shanshan Shi, Taiming Wei, Qi Wang,

Depression is a severe disabling psychiatric illness and the pathophysiological mechanisms remain unknown. In previous work, we found the changes in extrinsic coagulation (EC) pathway proteins in depressed patients compared with healthy subjects were significant. In this study, we screened differentially expressed proteins (DEPs) in the EC pathway, and explored the ... Read more >>

Bioengineered (Bioengineered)
[2021, 12(1):6318-6331]

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Direct Writing on Paper Substrate to Prepare Silver Electrode Structures for Flexible Sensors.

Qi Wang, Mingwei Li, Yao Xie, Yun Ou, Weiping Zhou,

With the rapid development of the electronics industry, electronic products based on silicon and glass substrates electronic products will gradually be unable to meet the rising demand. Flexibility, environmental protection, and low costs are important for the development of electronic products. In this study, an efficient and low-cost method for ... Read more >>

J Nanosci Nanotechnol (Journal of nanoscience and nanotechnology)
[2021, 21(12):6048-6053]

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Homeobox A5 activates p53 pathway to inhibit proliferation and promote apoptosis of adrenocortical carcinoma cells by inducing Aldo-Keto reductase family 1 member B10 expression.

Danyan Chen, Zhaonan Shen, Xi Cheng, Qi Wang, Junlin Zhou, Fang Ren, Yue Sun, Hongman Wang, Rongxi Huang,

Aldo-Keto Reductase Family 1 Member B10 (AKR1B10) and Homeobox A5 (HOXA5) are both down-regulated in adrenocortical carcinoma (ACC), and HOXA5 is predicted to bind to the promoter of AKR1B10. We aimed to investigate whether HOXA5 could bind to AKR1B10 to regulate ACC cells proliferation and apoptosis. The expression of AKR1B10 ... Read more >>

Bioengineered (Bioengineered)
[2021, 12(1):1964-1975]

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Antimicrobial photodynamic activity of gallium-substituted haemoglobin on silver nanoparticles.

Ana V Morales-de-Echegaray, Lu Lin, Badhu Sivasubramaniam, Aiganym Yermembetova, Qi Wang, Nader S Abutaleb, Mohamed N Seleem, Alexander Wei,

Methicillin-resistant Staphylococcus aureus (MRSA), a major scourge in skin and soft-tissue infections, expresses surface-bound haemoprotein receptors that can be exploited for the targeted delivery of photosensitizers. We have developed a nanosized agent for targeted antimicrobial photodynamic therapy (aPDT), comprised of GaPpIX (a hemin analog with potent photosensitizer activity) encapsulated in ... Read more >>

Nanoscale (Nanoscale)
[2020, 12(42):21734-21742]

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Evaluation and application of an efficient plant DNA extraction protocol for laboratory and field testing.

Qi Wang, Xiaoxia Shen, Tian Qiu, Wei Wu, Lin Li, Zhi'an Wang, Huixia Shou,

Nucleic acids in plant tissue lysates can be captured quickly by a cellulose filter paper and prepared for amplification after a quick purification. In this study, a published filter paper strip method was modified by sticking the filter paper on a polyvinyl chloride resin (PVC) sheet. This modified method is ... Read more >>

J Zhejiang Univ Sci B (Journal of Zhejiang University. Science. B)
[2021, 22(2):99-111]

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Clonal phylogeny and evolution of critical cytogenetic aberrations in multiple myeloma at single cell level by QM-FISH.

Yuting Yan, Xiaoqi Qin, Jiahui Liu, Huishou Fan, Wenqiang Yan, Lanting Liu, Chenxing Du, Zhen Yu, Yan Xu, Mu Hao, Shuhui Deng, Weiwei Wei Sui, Rui Lv, Wei Liu, Qi Wang, Dehui Zou, Linping Hu, Jianxiang Wang, Yu-Tzu Tai, Kenneth C Anderson, Lei Zhang, Tao Cheng, Anders Zetterberg, Nikhil C Munshi, Lugui Qiu, Gang An,

Single-cell analysis is of significant importance in delineate the exact phylogeny of subclonal population and in discovering subtle diversification. So far studies of intratumor heterogeneity and clonal evolution in multiple myeloma (MM) were largely focused at the bulk tumor population level. Here, we performed quantitative multi-gene fluorescence in situ hybridization ... Read more >>

Blood Adv (Blood advances)
[2021, :]

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Correlation of peripheral CD4+GranzB+CTLs with disease severity in patients with primary Sjögren's syndrome.

Qi Wang, Nan Che, Chengyin Lu, Xiaoxuan Sun, Yanyan Wang, Qiang Wang, Wenfeng Tan, Lanlan Zhou, Xiaojun Zhang, Dong Xu, Lei Gu, Miaojia Zhang,

<h4>Introduction</h4>Primary Sjögren's syndrome (pSS) is a chronic systemic autoimmune disease which has focal lymphocytic infiltration including a majority of CD4+ T cells. This study was to investigate the correlation of peripheral granzyme B (GranzB)-expressing CD4+ T cells with disease severity and histological lesion in patients with pSS.<h4>Methods</h4>We recruited 116 pSS ... Read more >>

Arthritis Res Ther (Arthritis research & therapy)
[2021, 23(1):257]

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Corrigendum to "RNA binding protein DAZAP1 promotes HCC progression and regulates ferroptosis by interacting with SLC7A11 mRNA".

Qi Wang, Yaxun Guo, Wentao Wang, Bingqi Liu, Guangsheng Yang, Zongzhen Xu, Jie Li, Zhiqian Liu,

Exp Cell Res (Experimental cell research)
[2021, :112867]

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Production of fermented spicy rabbit meat using Lactobacillus paracasei.

Xingxiu Zhao, Shilu Li, Yuanhao Liu, Yiguo He, Rong Hu, Jiao Yang, Qi Wang,

Lactobacillus paracasei was used to produce fermented spicy rabbit meat. A series of indexes were determined, including pH value, free amino acid content, true protein content, texture, microstructure and the volatile compounds of fermented spicy rabbit meat and unfermented spicy rabbit meat. The results showed that Lactobacillus paracasei could reduce ... Read more >>

Bioprocess Biosyst Eng (Bioprocess and biosystems engineering)
[2021, :]

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Morphological Changes of The Root Apex In Anterior Teeth With Periapical Periodontitis: An In-Vivo Study

Chen-chen Zhang, Ya-jing Liu, Wei-dong Yang, Qian-nan Zhang, Ming-zhu Zha, Shan-hui Wen, Qi Wang,

<h4>Introduction: </h4> The aim was to analyze the morphological changes of root apex in anterior teeth with periapical periodontitis. <h4>Methods: </h4>: 32 untreated anterior teeth with periapical periodontitis were enrolled, compared with the healthy contralateral teeth. Cone-beam computed tomography was used to measure diameter of the apical constriction. 3D reconstruction ... Read more >>

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A Regioselectively Oxidized 2D Bi/BiOx Lateral Nano-Heterostructure for Hypoxic Photodynamic Therapy.

Meng Qiu, Dou Wang, Hao Huang, Teng Yin, Wenli Bao, Bin Zhang, Zhongjian Xie, Ni Xie, Zongze Wu, Chenchen Ge, Qi Wang, Meng Gu, Hilliard L Kutscher, Liping Liu, Shiyun Bao, Paras N Prasad, Han Zhang,

Optoelectronic science and 2D nanomaterial technologies are currently at the forefront of multidisciplinary research and have numerous applications in electronics and photonics. The unique energy and optically induced interfacial electron transfer in these nanomaterials, enabled by their relative band alignment characteristics, can provide important therapeutic modalities for healthcare. Given that ... Read more >>

Adv Mater (Advanced materials (Deerfield Beach, Fla.))
[2021, :e2102562]

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Source-tracking of the Chinese Chikungunya viruses suggests that Indian subcontinent and Southeast Asia act as major hubs for the recent global spread of Chikungunya virus.

Shaofu Qiu, Jinpeng Guo, Peihan Li, Peng Li, Xinying Du, Rongzhang Hao, Chaojie Yang, Qi Wang, Hongbo Liu, Haoran Zhang, Sai Tian, Hua Shi, Liang Wen, Daizhi An, Xiaocui Yang, Xiaoyuan An, Ligui Wang, Changjun Wang, Hongbin Song,

<h4>Background</h4>Chikungunya fever, caused by the Chikungunya virus (CHIKV), has become a major global health concern, causing unexpected large outbreaks in Africa, Asia, Europe, and the Americas. CHIKV is not indigenous to China, and its origin in the country is poorly understood. In particular, there is limited understanding of the recent ... Read more >>

Virol J (Virology journal)
[2021, 18(1):203]

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A novel gene expression signature-based on B-cell proportion to predict prognosis of patients with lung adenocarcinoma.

Yi Zhang, Xuewen Yin, Qi Wang, Xuming Song, Wenjie Xia, Qixing Mao, Bing Chen, Yingkuan Liang, Te Zhang, Lin Xu, Feng Jiang, Xinyu Xu, Gaochao Dong,

<h4>Background</h4>This study aimed to develop a reliable immune signature based on B-cell proportion to predict the prognosis and benefit of immunotherapy in LUAD.<h4>Methods</h4>The proportion of immune cells in the TCGA-LUAD dataset was estimated using MCP-counter. The Least Absolute Shrinkage and Selector Operation was used to identify a prognostic signature and ... Read more >>

BMC Cancer (BMC cancer)
[2021, 21(1):1098]

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Tyrosine phosphatases regulate resistance to ALK inhibitors in ALK+ anaplastic large cell lymphoma.

Elif Karaca Atabay, Carmen Mecca, Qi Wang, Chiara Ambrogio, Ines Mota, Nina Prokoph, Giulia Mura, Cinzia Martinengo, Enrico Patrucco, Giulia Leonardi, Jessica Hossa, Achille Pich, Luca Mologni, Carlo B Gambacorti-Passerini, Laurence Brugieres, Birgit Geoerger, Suzanne D Turner, Claudia Voena, Taek-Chin Cheong, Roberto Chiarle,

Anaplastic large cell lymphomas (ALCLs) frequently carry oncogenic fusions involving the anaplastic lymphoma kinase (ALK) gene. Targeting ALK using tyrosine kinase inhibitors (TKIs) is a therapeutic option in cases relapsed after chemotherapy, but TKI resistance may develop. By applying genomic loss-of-function screens, we identified PTPN1 and PTPN2 phosphatases as consistent ... Read more >>

Blood (Blood)
[2021, :]

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A novel LRR-RLK (CTLK) confers cold tolerance through regulation on CBF pathway, antioxidants and proline accumulation.

Bohao Geng, Qi Wang, Risheng Huang, Yajie Liu, Zhenfei Guo, Shaoyun Lu,

Leucine-rich repeat-receptor-like kinase (LRR-RLK) is a large subfamily of plant RLKs, however, its roles in cold tolerance remain unknown. A novel cold tolerance LRR-RLK gene (MtCTLK1) in Medicago truncatula was identified using the transgenic lines overexpressing MtCTLK1 (MtCTLK1-OE) and mtctlk1 lines with Tnt1 retrotransposon insertion. Compared to the wild type ... Read more >>

Plant J (The Plant journal : for cell and molecular biology)
[2021, :]

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Relationship between hormonal contraceptives and sleep among women of reproductive age: a systematic review protocol.

Jinhui Ma, Megan Cheng, Lehana Thabane, Caihong Ma, Ning Zhang, Qi Wang, Hyunwoo Kim, Hameed Reza, Chunxue Wang, Xiaomei Yao,

<h4>Introduction</h4>The aetiology of sleep disruptions is unknown, but hormonal fluctuations during the menstrual cycle, pregnancy and menopause have been shown to potentially affect how well a woman sleeps. The aim of this systematic review was to investigate whether hormonal contraceptives are associated with a decreased quality of sleep and increased ... Read more >>

BMJ Open (BMJ open)
[2021, 11(10):e045819]

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A structural model of a Ras-Raf signalosome.

Venkatesh P Mysore, Zhi-Wei Zhou, Chiara Ambrogio, Lianbo Li, Jonas N Kapp, Chunya Lu, Qi Wang, Maxwell R Tucker, Jeffrey J Okoro, Gabriela Nagy-Davidescu, Xiaochen Bai, Andreas Plückthun, Pasi A Jänne, Kenneth D Westover, Yibing Shan, David E Shaw,

The protein K-Ras functions as a molecular switch in signaling pathways regulating cell growth. In the human mitogen-activated protein kinase (MAPK) pathway, which is implicated in many cancers, multiple K-Ras proteins are thought to assemble at the cell membrane with Ras effector proteins from the Raf family. Here we propose ... Read more >>

Nat Struct Mol Biol (Nature structural & molecular biology)
[2021, 28(10):847-857]

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